The Enhancement of CO2 Chemical Absorption by K2CO3 Aqueous Solution in the Presence of Activated Carbon Particles.pdfVIP

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The Enhancement of CO2 Chemical Absorption by K2CO3 Aqueous Solution in the Presence of Activated Carbon Particles.pdf

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The Enhancement of CO2 Chemical Absorption by K2CO3 Aqueous Solution in the Presence of Activated Carbon Particles.pdf

维普资讯 Chin．J．Chem．Eng．，15(6)842-- 846(2007) TheEnhancementofC02ChemicalAbsorptionbyK2CO3Aqueous SolutioninthePresenceofActivatedCarbonParticles LUSumin()~素敏)，MAYouguang(友光) ，ZHUChunying(朱春英)andSHENShuhua (沈树华) SchoolofChemicalEngineeringandTechnology，StateKeyLaboratoryofChemicalEngineering，TianjinUniver— sity,Tianjin300072，China Abstract Theenhnacementofchemi calabsorptionofCO，byK，CO1／H，O absorbentsinthepresenceofactivated crabonfAC、particleswasinvestigated．Theresultsshowthatthegasabsoprtionratescna beenhancedsignificantly inthepresenceofACparticles．na dthemaximum enhna cementfactor3．7wasobservedatlow stirringintensities． Theenhna cementfactorincreasedrapidlywiththesolidloadingduringtheinitialperiodofabsoprtionna dthenbe— camemi ldgraduallytoamxaimum value．Boththeliquid—solidcontactareana dtheprobabilityofsolidparticles residingatthegas—liquidinterfacedecreasedwiththeincreaseoftheparticlesize．1eadingtoanegativeeffectonthe enhna cementofmasstrna sfer,Theinfluenceoftheparticlesongasabsoprtiondecreasedwiththereactionrate．The stirringspeedchna gedtheinterfacialcoverageandmasstrna sferrateontheliquidsidena dconsequentlyaffected themasstrna sferbetweenthegasna dliquidphases；theenhna cementfactordecreasedwiththestirringintensity．A heterogeneoustwo—zonemodelwasproposedforpredicting theenhna cementfactorandthecalculatedresults agreedwellwiththeexperimentaldata． Keywords chemi calabsorption，enhancementfactor，masstrna sfer,activatedcrabonparticle 1 INTRoDUCTIoN Asthemaincontributortothegreenhouseeffect therecovery and rationalutilization ofCO7hasre— ceived considerableattention．Thechemicalabsorp— tion techniqueisusually employed in severalindus— trialprocesses，inwhichethanolamine1『，2】andpotas— sium carbonatesolvents3『，41asabsorbentsraecom— monly used．EthanolaminesfInainly monoethanola— mineanddietha