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Effect of 160 MeV Ni12+ ion irradiation on PbS quantum dots》.pdf
ARTICLE IN PRESS
Journal of Luminescence 114 (2005) 95–100
/locate/jlumin
Effect of 160 MeV Ni12+ ion irradiation on PbS quantum dots
a, a a b c
S. Chowdhury , D. Mohanta , G.A. Ahmed , S.K. Dolui , D.K. Avasthi ,
A. Choudhurya
aDepartment of Physics, Tezpur University, Napaam, Assam 784 028, India
bDepartment of Chemical Science, Tezpur University, Napaam, Assam 784 028, India
cNuclear Science Centre, Aruna Asaf Ali Marg, New Delhi 110 067, India
Received 17 August 2004
Available online 11 January 2005
Abstract
PbS quantum dots of average size 10 nm are encapsulated in a matrix (polyvinyl alcohol (PVA)) following chemical
12+ 12 13 2
route. They are irradiated with 160 MeV Ni ion beam with fluences 10 –10 ions/cm . Red shift in the absorption
response in the optical absorption spectra reveal size enhancement of the quantum dots after irradiation and was
confirmed by transmission electron microscopy (TEM). Photoluminescence (PL) study was carried out with excitation
wavelength 325 nm on both unirradiated and irradiated samples at different fluences and fluence-dependent surface
states and excitonic emission is observed in the PL study. The Huang–Rhys coupling constant decreases significantly
after swift heavy ion (SHI) irradiation and shows a decreasing tr
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