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A smart copper(II)-responsive binucleargadolinium(III) complex-based magnetic resonanceimaging contrast agent? Yan-meng Xiao,ab Gui-yan Zhao,ab Xin-xiu Fang,ab Yong-xia Zhao,ab Guan-hua Wang,c Wei Yang*a and Jing-wei Xu*a A novel Gd-DO3A-type bismacrocyclic complex, [Gd2(DO3A)2BMPNA], with a Cu2+-selective binding unitwas synthesized as a potential “smart” copper(II)-responsive magnetic resonance imaging (MRI) contrast agent. The relaxivity of the complex was modulated by the presence or absence of Cu2+; in the absence of Cu2+, the complex exhibited a relatively low relaxivity value (6.40 mM
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