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Clumped isotope thermometry of calcite and dolomite in a contact metamorphic environment.pdf

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Clumped isotope thermometry of calcite and dolomite in a contact metamorphic environment.pdf

Available online at ScienceDirect Geochimica et Cosmochimica Acta 197 (2017) 323–344 /locate/gca Clumped isotope thermometry of calcite and dolomite in a contact metamorphic environment Max K. Lloyd a,?, John M. Eiler a, Peter I. Nabelek b a Division of Geological and Planetary Sciences, California Inst. of Technology, Pasadena, CA 91125, United States b Department of Geological Sciences, University of Missouri, Columbia, MO 65211-1380, United States Received 23 March 2016; accepted in revised form 23 October 2016; available online 29 October 2016 Abstract Clumped isotope compositions of slowly-cooled calcite and dolomite marbles record apparent equilibrium temperatures of roughly 150–200 °C and 300–350 °C, respectively. Because clumped isotope compositions are sensitive to the details of T–t path within these intervals, measurements of the D47 values of coexisting calcite and dolomite can place new constraints on thermal history of low-grade metamorphic rocks over a large portion of the upper crust (from $5 to $15 km depth). We studied the clumped isotope geochemistry of coexisting calcite and dolomite in marbles from the Notch Peak contact metamorphic aureole, Utah. Here, ?at-lying limestones were intruded by a pluton, producing a regular, zoned metamorphic aureole. Calcite D47 temperatures are uniform, 156 ± 12 °C (2r s.e.), across rocks varying from high-grade marbles that exceeded 500 °C to nominally unmetamorphosed limestones 5 km from the intrusion. This result appears to require that the temperature far from the pluton was close to this value; an ambient temperature just 20 °C lower would not have permitted substantial re-equilibration, and should have preserved depositional or early diagenetic D47 values several km from the pluton. Combining this result with depth constraints from overlying strata suggests the country rock here had an average regional geotherm of 22.3–27.4 °C/km from the late Jurassic Period until at least the middle Paleogene Period. Dolo