Coupling system of AgBiOBr photocatalysis and direct contact membrane distillation for complete purification of N-containing dye wastewater.pdfVIP

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Coupling system of AgBiOBr photocatalysis and direct contact membrane distillation for complete purification of N-containing dye wastewater.pdf

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Coupling system of AgBiOBr photocatalysis and direct contact membrane distillation for complete purification of N-containing dye wastewater.pdf

Chemical Engineering Journal 317 (2017) 386–393 Contents lists available at ScienceDirect Chemical Engineering Journal journal homepage: /locate/cej Coupling system of Ag/BiOBr photocatalysis and direct contact membrane distillation for complete puri?cation of N-containing dye wastewater Rujing Hou a, Yuan Gao a, Huijuan Zhu a, Guoxiang Yang a, Wenhua Liu a, Yuning Huo a,?, Zongli Xie b,?, Hexing Li a,? a The Education Ministry Key Lab of Resource Chemistry, Shanghai Key Lab of Rare Earth Functional Materials, Shanghai Normal University, Shanghai 200234, China b CSIRO Manufacturing, Private Bag 10, Clayton South, VIC 3169, Australia highlights Photocatalysis-membrane reactor couples Ag/BiOBr ?lm and membrane distillation. Ag/BiOBr photodegrades picrolonic acid into CO2 and inorganic NH4+, NO2à and NO3à. Ag loading promotes visible-light absorbance and separates photoinduced charges. Membrane distillation produces clean water on permeate side by hydrophobicity. article info Article history: Received 18 December 2016 Received in revised form 14 February 2017 Accepted 16 February 2017 Available online 20 February 2017 Keywords: Photocatalytic membrane reactor (PMR) Visible-light Ag/BiOBr photocatalytic ?lm Direct contact membrane distillation (DCMD) Inorganic nitrogen species from picrolonic acid (PC) degradation Complete puri?cation of wastewater graphical abstract abstract A novel photocatalysis-membrane reactor (PMR) is designed by coupling Ag/BiOBr visible-light photocatalysis with thermal driven membrane distillation. Ag/BiOBr ?lms coated on glass substrates in a thin rectangular wastewater tank could avoid light-shielding effect from color solution containing dyepollutant. Meanwhile, Ag-modi?cation promotes the photocatalysis process owing to both the plasma effect and electric conductivity, which could enhance absorbance capability for visible lights and facilitate the separation of photo-induced electrons from holes to inhibit their recombination. When