CLEO会议激光脉冲堆积CLEO会议激光脉冲堆积.pdfVIP

Enhancement of spectral resolution and accuracy in asynchronous-optical-sampling terahertz time-domain spectroscopy for low- pressure gas-phase analysis Takeshi Yasui,1,2,* Kohji Kawamoto,1 Yi-Da Hsieh,1 Yoshiyuki Sakaguchi,1 Mukesh Jewariya,2 Hajime Inaba,3 Kaoru Minoshima,3 Francis Hindle,4 and Tsutomu Araki1 1Graduate School of Engineering Science, Osaka University, 1-3 Machikaneyama, Toyonaka, Osaka 560-8531, Japan 2Institute of Technology and Science, The University of Tokushima, 2-1 Minami-Josanjima, Tokushima, Tokushima 770-8506, Japan 3National Metrology Institute of Japan, National Institute of Advanced Industrial Science and Technology, 1-1-1 Umezono, Tsukuba, Ibaraki 305-8563, Japan 4 Laboratoire de Physico-Chimie de lAtmosphère, Université du Littoral C?te dOpale, 189A Av. Maurice Schumann, Dunkerque 59140, France *yasui@me.tokushima-u.ac.jp Abstract: The spectral resolution and accuracy of asynchronous-optical- sampling terahertz time-domain spectroscopy (ASOPS-THz-TDS) were evaluated by examining low-pressure gas-phase samples. Use of dual 56- MHz, erbium (Er)-doped, mode-locked femtosecond fiber lasers enhanced the spectral resolution to as low as 50.5 MHz and the spectral accuracy to as low as 6.2 × 10?6. The results indicate that ASOPS-THz-TDS has the potential to achieve high spectral resolution, high spectral accuracy, and wide spectral coverage at the same time. ASOPS-THz-TDS will open a new door to gas-phase spectroscopy of multiple chemical species in the field of atmospheric gas analysis. ?2012 Optical Society of America OCIS codes: (120.6200)