Two-Photon Polarization Dependent Spectroscopy in Chirality A Novel Experimental-Theoretical Approach to Study Optically Active Systems 英文参考文献.docVIP

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Two-Photon Polarization Dependent Spectroscopy in Chirality A Novel Experimental-Theoretical Approach to Study Optically Active Systems 英文参考文献.doc

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Two-Photon Polarization Dependent Spectroscopy in Chirality A Novel Experimental-Theoretical Approach to Study Optically Active Systems 英文参考文献

Molecules 2011, 16, 3315-3337; doi:10.3390/moleculeOPEN ACCESS molecules ISSN 1420-3049 /journal/molecules Review Two-Photon Polarization Dependent Spectroscopy in Chirality: A Novel Experimental-Theoretical Approach to Study Optically Active Systems Florencio E. Hernández 1,2 and Antonio Rizzo 3,* 1 Department of Chemistry, University of Central Florida, P. O. Box 162366, Orlando, FL 382616, USA 2 The College of Optics and Photonics, CREOL University of Central Florida, P. O. Box 162366, Orlando, FL 382616, USA 3 Consiglio Nazionale delle Ricerche (CNR), Istituto per i Processi Chimico Fisici (IPCF-CNR), UoS di Pisa, Area della Ricerca, Via G. Moruzzi 1, I-56124 Pisa, Italy * Author to whom correspondence should be addressed; E-Mail: rizzo@r.it; Tel.: +39-050-315-2456; Fax: +39-050-315-2442. Received: 2 March 2011; in revised form: 7 April 2011 / Accepted: 12 April 2011 / Published: 18 April 2011 Abstract: Many phenomena, including life itself and its biochemical foundations are fundamentally rooted in chirality. Combinatorial methodologies for catalyst discovery and optimization remain an invaluable tool for gaining access to enantiomerically pure compounds in the development of pharmaceuticals, agrochemicals, and flavors. Some exotic metamaterials exhibiting negative refractive index at optical frequencies are based on chiral structures. Chiroptical activity is commonly quantified in terms of circular dichroism (CD) and optical rotatory dispersion (ORD). However, the linear nature of these effects limits their application in the far and near-UV region in highly absorbing and scattering biological systems. In order to surmount this barrier, in recent years we made important advancements on a novel non linear, low-scatter, long-wavelength CD approach called two-photon absorption circular dichroism (TPACD). Herein we present a descriptive analysis of the optics principles behind