Electrical Conductivity Response of Poly(Phenylene-vinylene) Zeolite Composites Exposed to Ammonium Nitrate.docVIP

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Electrical Conductivity Response of Poly(Phenylene-vinylene) Zeolite Composites Exposed to Ammonium Nitrate.doc

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Electrical Conductivity Response of Poly(Phenylene-vinylene) Zeolite Composites Exposed to Ammonium Nitrate

Sensors 2010, 10, 5590-5603; doi:10.3390/s100605590 OPEN ACCESS sensors ISSN 1424-8220 /journal/sensors Article Electrical Conductivity Response of Poly(Phenylene-vinylene)/ Zeolite Composites Exposed to Ammonium Nitrate Jirarat Kamonsawas 1, Anuvat Sirivat 1,*, Sumonman Niamlang 2, Pimpa Hormnirun 3 and Walaiporn Prissanaroon-Ouajai 4 1 Center of Excellence in Petroleum Petrochemicals and Advanced Materials, The Petroleum and Petrochemical College, Chulalongkorn University, Soi Chula 12, Phayathai Road, Phatumwan, Bangkok, 10330, Thailand; E-Mail: som_news@ (J.K.) 2 Department of Materials and Metallurgical Engineering, Faculty of Engineering, Rajamangala University of Technology Thanyaburi, Rangsit-Nakhonnayok Road, Klong 6, Thanyaburi, Phatumthani, 12110, Thailand; E-Mail: tanggggo@ (S.N.) 3 Department of Chemistry, Faculty of Science, Kasetsart University, 50 Phahonyothin Road, Ladyao, Chatuchak, Bangkok, 10900, Thailand; E-Mail: fscipph@ku.ac.th (P.H.) 4 Department of Industrial Chemistry, Faculty of Applied Science, KMIT-NB, 1518 Pibulsongkram Road, Bangsue, Bangkok, 10800, Thailand; E-Mail: pwalaip@ (W.P.-O.) * Author to whom correspondence should be addressed; E-Mail: anuvat.s@chula.ac.th; Tel.: +66-2-218-4131; Fax: +66-2-611-7221. Received: 30 January 2010; in revised form: 27 March 2010 / Accepted: 22 April 2010 / Published: 3 June 2010 Abstract: Poly(p-phenylenevinylene) (PPV) was chemically synthesized via the polymerization of p-xylene-bis(tetrahydrothiophenium chloride) monomer and doped with H2SO4. To improve the electrical conductivity sensitivity of the conductive polymer, Zeolites Y (Si/Al = 5.1, 30, 60, 80) were added into the conductive polymer matrix. All composite samples show definite positive responses towards NH4NO3. The electrical conductivity sensitivities of the composite sensors increase linearly with increasing Si/Al ratio: with values of 0.201, 1.37, 2.80 and 3.18, re