原创力文档conducting polymers functionalized with phthalocyanine as nitrogen dioxide sensors导电聚合物功能化与酞菁二氧化氮传感器.pdfVIP
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conducting polymers functionalized with phthalocyanine as nitrogen dioxide sensors导电聚合物功能化与酞菁二氧化氮传感器
Sensors 2002, 2, 185-194
sensors
ISSN 1424-8220
© 2002 by MDPI
/sensors
Conducting Polymers Functionalized with Phthalocyanine as
Nitrogen Dioxide Sensors
S.Radhakrishnan* and S.D.Deshpande
Polymer Science Engineering, National Chemical Laboratory, Pune- 411008 (India)
* Author to whom correspondence should be addressed. E-mail: srr@ems.ncl.res.in
Received:18 April 2002 / Accepted: 10 May 2002 / Published: 15 May 2002
Abstract: The conducting polymers such as polyaniline, polypyrrole and polythiophene
were functionalized with copper phthalocyanine using chemical oxidation method. The
obtained polymers viz. PANI-CuPc, PPy-CuPc and PT-CuPc were studied as chemical
sensors by their response characteristics after exposure to various chemical vapors such as
methanol, ammonia and nitrogen dioxide. The results obtained showed that these polymers
have moderate sensitivity towards the methanol as well as ammonia vapors whereas they
show tremendous sensitivity towards nitrogen dioxide vapors. The sensitivity factor of as
high as 50,000 was obtained for PT-CuPc polymers in nitrogen dioxide. In comparison to
this, the sensitivity factors of about 100 and 40 were obtained, when these polymers were
exposed to ammonia and methanol vapors. The very high selectivity towards the nitrogen
dioxide was explained on the basis of charge transfer complex formed
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