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occurrence, biological activities and synthesis of kaurane diterpenes and their glycosides发生、生物活性和合成kaurane二萜及其苷类.pdf

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occurrence, biological activities and synthesis of kaurane diterpenes and their glycosides发生、生物活性和合成kaurane二萜及其苷类

Molecules 2007, 12, 455-483 molecules ISSN 1420-3049 Review Occurrence, Biological Activities and Synthesis of Kaurane Diterpenes and their Glycosides Pablo Anselmo García 1, Alaíde Braga de Oliveira 2 and Ronan Batista 3,* 1 Departamento de Química Farmacéutica, Facultad de Farmacia, Universidad de Salamanca, Campus Miguel de Unamuno, 37007 Salamanca, Spain; E-mail: pabloagg@usal.es 2 Departamento de Produtos Farmacêuticos, Faculdade de Farmácia, Universidade Federal de Minas Gerais, Av. Antônio Carlos, 6627, 31270-901 Belo Horizonte – MG, Brazil; E-mail: alaidebraga@.br 3 Departamento de Estudos Básicos e Instrumentais, Universidade Estadual do Sudoeste da Bahia, BR 415, Km 03, s/nº, 45.700-000 Itapetinga – BA, Brazil * Author to whom correspondence should be addressed; E-mail: ronbatis2004@. Received: 18 February 2007; in revised form: 12 March 2007 / Accepted: 12 March 2007 / Published: 13 March 2007 Abstract: This paper presents a review on kaurane diterpenes and their glycoside derivatives, covering aspects of their occurrence, biological activities and the synthesis of these natural products and their analogues. First, it shows and classifies diterpenes, in accordance with the already established structural criteria in the literature. Then, kaurane diterpenes are presented, focusing on their chemical structures, occurrence in the plant kingdom and their main, recently described, biological activities. Moreover, the most significant works, published between 1964 and November 2006, which describe the total synthesis or structur