原创力文档reduction–oxidation photocycle dynamics of flavins in starch filmsreduction-oxidation photocycle动力学淀粉黄素的电影.pdfVIP
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reduction–oxidation photocycle dynamics of flavins in starch filmsreduction-oxidation photocycle动力学淀粉黄素的电影
Int. J. Mol. Sci. 2012, 13, 9157-9183; doi:10.3390/ijm
OPEN ACCESS
International Journal of
Molecular Sciences
ISSN 1422-0067
/journal/ijms
Article
Reduction–Oxidation Photocycle Dynamics of Flavins in
Starch Films
Alfons Penzkofer
Faculty of Physics, University of Regensburg, Universitaetsstrasse 31, D-93053 Regensburg,
Germany; E-Mail: alfons.penzkofer@physik.uni-regensburg.de; Tel.: +49-941-943-2107;
Fax: +49-941-943-2754
Received: 10 May 2012; in revised form: 2 July 2012 / Accepted: 11 July 2012 /
Published: 23 July 2012
Abstract: The blue-light photo-reduction (conversion of oxidized flavin quinone via flavin
semiquinone to fully reduced flavin hydroquinone) and dark re-oxidation of the flavins
riboflavin and lumiflavin in starch (α-amylose) films was studied by absorption and
luminescence spectroscopy. Blue-light photo-excitation caused an absorption, fluorescence,
and phosphorescence decrease which recovered in the dark. The photo-reduction
dark-oxidation cycle could be repeated. The efficiency of photo-reduction decreased with
exposed excitation energy, and the speed of re-oxidation in the dark slowed down with
time after excitation. The absorption did not fully recover. The fluorescence efficiency
after a long time of storage in the dark increased
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