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Apr.2010,Volume4,No.4(SerialNo.29)
JournalofMaterialsScienceandEngineering,ISSN 1934—8959,USA 《
Low FrreeqquueennccYyDDispeerrssioonnlinIIonicConductionooft
(1-x)(Nal一4Ag1)一xAI20s
LuisAlrfedoRodriguezGonzalez,WilmerBuchelli,HernandoCorrea,JesfisE.Diosa andRub6nAntonio
VargasZapata
, GrupodeTransicionesdeFaseenSistemasnoM et6licos.UniversidaddelValle,A.A.25360Cali,Colombia
2.InstitutodeCienciadeMaterialesdeMadrid,CSIC,Cantoblanco28049,Madrid,Espaha
3.Laboratoriode Optoelectr6nica,UniversidaddelQuindio,Armenia。Colombia
Received:December01,2009/Accepted:December28,2009/Published:April25,2010
Abstract:Inthispaper,theauthorsinvestigatethetemperaturedependenceofthelongrangeioniccorrelationinthehighlydisordered
structureofthe(1一x)(Nal一4Ag1)一x(AI2O3)(x=0.1,0.2and0.3)compositesbyadmittancemeasurementsintheaudiorfequencyrange
Anon—Arrheniusbehaviorisobservedinthetemperature(T)dependenceoftherealpartoftheconductivity,13-’,thatcanbewellfitted
totheexpressionlog(~)‘=exp[·((1000/一,) +C,wherekl,如andCarefittingparametersthatdependonthealuminacontentand
therfequencyresponsebehaviorofconductivityinthevariousdispersiveregionswithidenticalshapeofthespectra.Theobservedwell
definedlow rfequencydispersionbehaviorof仃’,particularlyattemperaturesbelow thesuperionictransitionofAglat470K,is
consistentwiththegranularmorphologyofthematerialandthehighly correlated hoppingionicmotion inthebulkofitsionic
conductinggrainsandacrosstheinterfacebetweenitscomponents.
Keywords:Ionicconductivity Ag1.composite,non—arrhenius
1.IntrOductiOn glasses,polymers,ioniccrystalsathighrfequencies,(o
2兀厂(Hz),suchthattherealpartoftheelectrical
ThedynamicsofmobileIonsincondensedmatter
conductivitycanbedescribedby[5]
areofspecialinterestsincethey arerelatedto ionic
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