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专题之动力学光谱激光化学和光化学动力学类
墙贴摘要正文
专题之三、动力学光谱、激光化学和光化学动力学类
P3-70
An efficient quantum approach for studying the interaction
of atoms and circularly polarized laser fields
Minghu Yuan, Tianshu Chu, Keli Han*
State Key Laboratory of Molecular Reaction Dynamics, Dalian Institute of Chemical Physics,
Chinese Academy of Sciences, Dalian, 116023, China
We present anefficient quantum approach for exploring physical processes of various atomic targets
interacting with strong circularly polarized laser fields, based on thesine-DVR method[1, 2] which is
high-efficiency and accurate for studying the interaction of atoms/molecules and linearly polarized laser
fields.However, the sine-DVR method is helpless when atoms/molecules exposed in circularly polarized
laser fields.
In this work, we introduceWigner rotation in the time propagation due to the circularly polarized light
can be deemed to the rotation of linearly polarized light with time. We determine the interactions of
electron with nuclei and field in laboratory fixed coordinate system, respectively.Every step can be split
into three sub-steps.Firstly, we assume that the atoms/molecules main axis is parallel with the zaxis and the
polarization direction of laser is arbitrary. Then we can calculate the interaction of electron with nuclei.
Secondly, we transform the electron wave function with the Wigner rotation matrix making that the
polarization direction of laser is parallel with the z axis. So, we can calculate the interaction of electron
with field. Thirdly, we can return to the electron wave function by the inverse rotation, and calculate the
interaction of electron and nuclei.The processes are showi
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