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化学计量学在遥感FTIR谱图解析中的应用及发展-化学工程与技术专业论文
博士论文
博士论文 化学计量学在遥感FTIR谱图解析中的应用及发展
Abstract
Techniques were set up in the dissertation with the aid of chemometrics,which were used for interpretation on remote sensing FTIR spectrum of VOCs(volatile organic compounds)in the atmosphere.These especially strengthen the advantage of
remote sensing F11R in quick,accurate.real.time and simultaneous determination of
multi-component analysis.Since the remote sensing FTIR spectrum containing much noise,unknown interferents and background shift,strategies were put forward in the
viewpoint of model robust and popularity.Based on the multivariate calibration method PLS(pardal least squares),new signal correction method OSC(orthogonal signal correction)was applied to the filtration of noise or other unrelated parts and good performance was yielded in model simplicity and robust.Furthermore,PLS were improved in the direction of inner relation with the use of PPLS(polynomial partial least squares)model and Were employed in the five-component mixture successfully.Calibration transfer was applied innovatively in the analysis of the remote sensing FTIR spectrum.With the optimization ofthis method,remote sensing
FTIR spectra were analyzed directly with EPA spccR'a.PLS Was also used for the
pattern recognition of VOCs,and qualitative and quantitative analysis were achieved simultaneously with the help of experiment design.Prima巧interpretation of passive remote sensing FTIR SpP戈ql"Bl'n Was carried out.The innovation-application of
PARAFAC(parallel factor analysis)Was utilized for the analysis of passive remote sensing FTIR spectrlml and qualitative and quantitative analyses were realized.The main conclusions Were achieved as following:
1.Interpretation Oil Remote Sensing FTIR Spectrum Based On PLS
According to the signal characteristics of remote sensing FTIP、,PLS Was improved in the viewpoint of model popularity and robust.As for the remote锄塔ing F1]喂data,noise in the data enlarged the L
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