Physicochemical and Interfacial Investigation of Lipid Polymer Particle Assemblies英文文献资料.pdfVIP

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Physicochemical and Interfacial Investigation of Lipid Polymer Particle Assemblies英文文献资料.pdf

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Langmuir 2005, 21, 1305 Physicochemical and Interfacial Investigation of Lipid/ Polymer Particle Assemblies Anne-Lise Troutier, Thierry Delair, Christian Pichot, and Catherine Ladavie`re* UMR 2714 CNRS/bioMe´rieux, Syste`mes Macromole´culaires et Physiopathologie Humaine, ENSL, 46, alle´e dItalie, 69364 Lyon Cedex 07, France Received September 20, 2004. In Final Form: November 2, 2004 A model study was investigated to develop colloidal supramolecular assemblies consisting of particles coatedwithlipidlayers.Theinteractionsbetweenmonodispersesulfate-chargedpoly(styrene)submicrometer particles and zwitterionic/cationic lipid vesicles composed of 1,2-dipalmitoyl-sn-glycero-3-phosphocholine and 1,2-dipalmitoyl-3-trimethylammonium propane were considered. The influence of relevant experimental parameters on the final associations was examined by quasi-elastic light scattering to point out some new phenomena occurring in these colloidal systems. The major role of electrostatic interactions as driving forces to control the organization between cationic lipids and oppositely charged poly(styrene) particles was clearly evident, whereas this influence was less pronounced when considering the zwitterionic lipids. The characterization of these original complex assemblies was completed by a thorough study of the surface modification. The combination of zeta potential measurements, X-ray photoelectron spectroscopy analyses, and microscopy observations proved that the envisioned model can really correspond to polymer