不同特征污染源中指示性药物和个人护理品识别与筛选.pdf

中国环境科学 2019,39(3) ：1173~1180 China Environmental Science 不同特征污染源中指示性药物和个人护理品识别与筛选 * 梅雪冰,隋 倩 ,张紫薇,姚根吉,何梦达,陈智翀, 吕树光 (华东理工大学资源与环境工程学院, 国家环境保护化工过程 环境风险评价与控制重点实验室,上海 200237) 摘要：通过分析我国地表水中药物和个人护理品(PPCPs)主要污染源排放特征,识别和筛选出咖啡因、卡马西平和磺胺嘧啶为我国地表水环境中的指示 性 PPCPs(i-PPCPs),分别指征城镇生活污水、城镇污水处理厂出水和养殖废水三类特征污染排放源.同时,基于筛选的 i-PPCPs 开展了初步应用研究,结 果表明,生活污水是北运河和黄浦江流域地表水中 PPCPs 的主要来源.研究结果为构建更综合和有效的 PPCPs 的溯源体系,识别我国城市地表水环境中 PPCPs 的主要排放源提供了理论依据. 关键词：药物和个人护理品；指示性药物和个人护理品；特征污染源；溯源 中图分类号：X522 文献标识码：A 文章编号：1000-6923(2019)03-1173-08 Identification of indicator pharmaceutical and personal care products (PPCPs) in different emission sources. MEI Xue-bing, * SUI Qian , ZHANG Zi-wei, YAO Gen-ji, HE Meng-da, CHEN Zhi-chong, LÜ Shu-guang (State Environmental Protection Key Laboratory of Environmental Risk Assessment and Control on Chemical Process, School of Resource and Environmental Engineering, East China University of Science and Technology, Shanghai 200237, China). China Environmental Science, 2019,39(3) ：1173~1180 Abstract ：In the present study, caffeine, carbamazepine and sulfadiazine were identified as indicator PPCPs (i-PPCPs) in the surface water environment of China, which indicated the typical emission sources of domestic wastewater, effluent of municipal wastewater treatment plants and livestock wastewater, respectively. Then, the identified i-PPCPs were used for a preliminary source apportionment of PPCPs in the urban water environments. The results indicated that domestic wastewater was the main source of PPCPs in the surface water of Beiyun River in Beijing and Huangpu River in Shanghai. The findings provide a theoretical basis for building a more comprehensive and effective source apportionment system of PPCPs and identifying the main sources of PPCPs in urban surface water environment in China. Key