含咪唑基配体钛锆金属配合物的合成及催化性能研究的中期报告.docxVIP

含咪唑基配体钛锆金属配合物的合成及催化性能研究的中期报告 摘要 本中期报告针对含咪唑基配体的钛锆金属配合物的合成方法进行了研究，并考察了配合物的催化性能。首先，我们合成了两种不同结构的含咪唑基配体，并通过核磁共振、质谱和元素分析等手段对其结构进行了表征。随后，我们将合成得到的该配体与钛或锆氯化物反应，获得了不同金属配合物。通过红外光谱、核磁共振和元素分析等手段，对配合物的结构进行了表征。最后，我们将配合物用于不同的催化反应中进行了研究，考察了其催化性能。 关键词：咪唑基配体，钛锆金属配合物，合成 method，催化性能 Abstract This midterm report focuses on the synthesis of titanium-zirconium metal complexes containing imidazole-based ligands and investigates their catalytic properties. Firstly, we synthesized two different structures of imidazole-based ligands and characterized their structures by nuclear magnetic resonance, mass spectrometry and elemental analysis. Subsequently, we reacted the obtained ligand with titanium or zirconium chloride to obtain different metal complexes. The structure of the complex was characterized by infrared spectroscopy, nuclear magnetic resonance and elemental analysis. Finally, we studied the catalytic performance of the complexes in different catalytic reactions. Keywords: imidazole-based ligand, titanium-zirconium metal complex, synthesis method, catalytic properties.