英文合成高性能防污膜聚醚砜纳滤膜去除废水中的颜色.pdf

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EnvironmentalScienceandPollutionResearch(2022)29:20463–20478

/10.1007/s11356-021-16655-8

RESEARCHARTICLE

Colorremovalfromwastewaterusingasynthetichigh-performance

antifoulingGO-CPTMS@Pd-TKHPP/polyethersulfone

nanofiltrationmembrane

FoadGholami1SirusZinadini1SoheilaNakhjiriKamrani2AliAkbarZinatizadeh1,3KiumarsBahrami2,4

Received:31May2021/Accepted:17September2021/Publishedonline:5November2021

#TheAuthor(s),underexclusivelicencetoSpringer-VerlagGmbHGermany,partofSpringerNature2021

Abstract

Modifiedgrapheneoxidewith5,10,15,20-tetrakis-(4-hexyloxyphenyl)-porphyrinandpalladium(II)(signifiedbyGO-

CPTMS@Pd-TKHPP)preparedasanovelantifoulingpolyethersulfone(PES)blendednanofillermembrane.Themembrane

efficiencyhasbeenanalyzedsuchaspurewaterflux(PWF),hydrophilicity,andantifoulingfeatures.Byincreasingofmodified

grapheneoxidepercentagefrom0to0.1wt.%inthepolymermatrix,thePWFwasincrementedfrom14.35to37.33kg/m2·hat4

bar.Themembranefluxrecoveryratio(FRR)hasbeeninvestigatedbyapplyingpowderedmilksolution;theFRRresults

indicatedthatthe0.1wt.%-modifiedgrapheneoxidemembraneshowedapositiveeffectonfoulingbehaviorwithRirand

FRRvalue8.24%and91.76%,respectively.ThenanofiltrationmembraneperformancewasassessedapplyingtheDirectRed16

dyerejection.Itwasdemonstratedthattheoptimalmembranes(0.1wt.%-modifiedgrapheneoxide)hadnotabledyeremoval

(99.58%rejection).Theresultsarealsoverifiedbymeasuringthescanningelectronmicroscopy(SEM),watercontactangle

(WCA),andatomicmicroscopyanalysis(AFM).

KeywordsPolyethersulfone.Nanofiltrationmembrane.Antifoulingproperty.Modifiedgrapheneoxide.Dyeremoval.

Wastewatertreatment

Introductiontreatedbeforewastewaterdrainsintotheenvironment(tor

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