《g-C3N4三元复合光催化剂的制备及其可见光驱动下的光催化活性增强.》.pdf

ChineseJournalofCatalysis35(2014)78—84 催化学报 2014年 第35卷 第1期 1www．chxb．cn Article PreparationofternaryAg／Ag3PO4／g-C3N4hybridph0tocatalystsand theirenhancedphotocatalyticactivitydrivenbyvisiblelight KaiShena ，MohammedAshrafGondalb，-．，RashidGhulam Siddiqueb，ShanShiaSiqiWanga， IiangboSunanQingyuXu CollegeofMaterialsScienceandTechnology,NanjingUniversityofAeronauticsandAstronautics,Nanjing211100,]iangsu,China LaserResearchGroup,PhysicsDepartmentandCenterofExcellenceinNanotechnology,骼哪FahdUniversiytofPetroleumandMinerals,Dhahran 31261SaudiArabia cDepartmentofPhysics,SoutheastUniversity,Nanjina2n189，ndngsu’China A R T IC L E IN F 0 A B ST R A C T Articlehistory： ThepreparationofaseriesofternaryAg／Ag3PO4／g-C3N4hybridphotocatalystswhichdisplayen- Received26July2013 hancedphotocatalyticactivity，wasreported，Thecrystalstructure，morphology，composition，opti— Accepted10September2013 calabsorption，andefficientseparationofchargecarrierswerestudiedbyX—raydiffraction，scan— Published20January2014 ningelectronmicroscopy,absorptionandphotoluminescencespectroscopymeasurements．Using rhodamineBasamodelcontaminant,theasp·reparedAg／Ag3PO4／gC·3N4hybridphotocaatlyst exhibitedsuperiordegradationperformanceundervisiblelightirradiationthanAg3P04orbinary Keywords： Silvernanoparticle AgaPO4／g-C3N4hybridphotocatalystsystems．Thesurfaceplasmonresonanceofthe4Onm-silver nanoparticlesformedonthesurfaceofAg3P04andtheheterojunctionformedattheinterfacebe- Silverorthophosphate(Ag3P04) tweenAg3P04andg-C3N4，areconsideredtobehtemajorphysical·chemicaloriginandtoberespon- Graphiticcarbonnitride -C3N4)