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MECHANIAL, DIELECTRIC AND ACTUATED STRAIN OF SILICONE ELASTOMER FILLED
Mechanical, dielectric and actuated strain of silicone elastomer filled with various types of TiO2
Haoliang Liu,1 Liqun Zhang,1,2 Dan Yang,1 Yingchun Yu,1,2 Lu Yao1, and Ming Tian1,2*
1Key Laboratory of the Preparation and Processing of Novel Polymer Materials, Beijing University of Chemical Technology, Beijing, China 100029
2State Key Laboratory of Organic-Inorganic Composites, Ministry of Science and Technology, Beijing, China 100029
Address: Beijing University of Chemical Technology, NO.15 Of North Three-ring East Road, Chao Yang District, BEIJING, CHINA
Email: tian71402@126.com; ilovetbag@163.com
Mechanical, dielectric, and actuated strain of silicone elastomer filled with various types of TiO2
This paper presents a comprehensive study of the effects of titanium dioxide (TiO2) on the dielectric, mechanical and electromechanical properties of a dielectric elastomer. The dielectric elastomer films, consisting of a high breakdown voltage silicone matrix in which different grain sizes of rutile form and nanometer of mixed crystal form of TiO2 particles were dispersed, were fabricated by casting and vulcanization at room temperature. The studied silicone/TiO2 composite film exhibited, in comparison with pure silicone, a steadily improvement of dielectric constant and elastic modulus with the augment of TiO2 particles. A transverse planar strain of 18% with pre-strain of 5% at 50V/μm was obtained, which was 50% higher than the corresponding value generated with the pure silicone. The practical actuated strain was lower than the theoretical, and it was well explained. The actuated strain of dielectric elastomer was not only closely related to dielectric constant and elastic modulus, but also to mechanical and dielectric loss. The nano-TiO2 could not provide higher dielectric than macro-TiO2 in the case of relatively poor dispersion. In consideration of the equilibrium of dielectric properties and mechanical properties, the micron fillers can improve the actuated str
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