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4.Advanced Materials-All-Solid-State Flexible Ultrathin Micro-Supercapacitors Based on Graphene.pdf

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4.Advanced Materials-All-Solid-State Flexible Ultrathin Micro-Supercapacitors Based on Graphene

www.advmat.de www.MaterialsV C O M M U N IC A Zhiqiang Niu , Li Zhang , Lili Liu , Bowen Zhu , Haibo Dong , and Xiaodong Chen * All-Solid-State Flexible Ultrathin Micro-Supercapacitors Based on Graphene TIO N The recent boom in portable electronic devices has raised the demand for power sources which are suffi ciently compact and can potentially be integrated on a fl exible chip with other electronic components. [ 1 ] In addition, miniaturizing energy storage devices onto a chip would potentially increase the den- sity of devices with different functionalities and reduce overall chip design complexity by removing intricate interconnects to bulk-sized energy storage devices. [ 2 ] Supercapacitors are an important class of energy storage devices which have attracted signifi cant attention because of their higher power density, cycle effi ciency, and charge/discharge rates as against batteries. [ 3–28 ] Recent work has illustrated that high performance micro-scale supercapacitors can be fabricated onto a chip using different active materials and designs, such as carbon nanotubes (CNTs), activated carbons, and conductive polymers. [ 1 , 2 , 29–38 ] As a fundamental two-dimensional material, graphene sheets have been used as basic building blocks to construct graphene-based structures for use as supercapacitor elec- trodes. [ 7–9 , 39–41 ] Since microelectrodes with 2D permeable chan- nels are required for integrating micro-supercapacitors on a substrate, graphene sheets are ideally suited to construct micro- supercapacitor electrodes by virtue of their unique 2D struc- ture and exceptional properties, such as high in-plane electrical conductivity and large specifi c surface area. [ 42 ] For example, graphene-based micro-supercapacitors have been fabricated on graphene oxide (GO) paper by direct laser writing, [ 43 ] and micro- supercapacitors using micro-patterned interdigitated electrodes composed of reduced GO (rGO) and CNT composi