Bactericidal Performance of Visible-Light Responsive Titania Photocatalyst with Silver Nanostructures 英文参考文献.docVIP

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Bactericidal Performance of Visible-Light Responsive Titania Photocatalyst with Silver Nanostructures 英文参考文献.doc

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Bactericidal Performance of Visible-Light Responsive Titania Photocatalyst with Silver Nanostructures 英文参考文献

BactericidalPerformanceofVisible-LightResponsive TitaniaPhotocatalystwithSilverNanostructures Ming-ShowWong1,2.,Der-ShanSun3.,Hsin-HouChang2,3,4 * 1DepartmentofMaterialsScienceandEngineering,NationalDong-HwaUniversity,Hualien,Taiwan,2NanotechnologyResearchCenter,NationalDong-HwaUniversity, Hualien,Taiwan,3DepartmentofMolecularBiologyandHumanGenetics,Tzu-ChiUniversity,Hualien,Taiwan,RepublicofChina,4Tzu-ChiUniversityCenterforVascular Medicine,Tzu-ChiUniversity,Hualien,Taiwan,RepublicofChina Abstract Background:Titaniadioxide(TiO2)photocatalystisprimarilyinducedbyultravioletlightirradiation.Visible-lightresponsive anion-doped TiO2 photocatalysts contain higher quantum efficiency under sunlight and can be used safely in indoor settings without exposing to biohazardous ultraviolet light. The antibacterial efficiency, however, remains to be further improved. Methodology/PrincipalFindings:Usingthermalreductionmethod,herewesynthesizedsilver-nanostructurescoatedTiO2 thinfilmsthatcontainahighvisible-lightresponsiveantibacterialproperty.Amongourtestedtitaniasubstratesincluding TiO2,carbon-dopedTiO2[TiO2(C)]andnitrogen-dopedTiO2[TiO2(N)],TiO2(N)showedthebestperformanceaftersilver coating.Thesynergisticantibacterialeffectresultsapproximately5logreductionsofsurvivingbacteriaofEscherichiacoli, Streptococcus pyogenes, Staphylococcus aureus and Acinetobacter baumannii. Scanning electron microscope analysis indicated that crystalline silver formed unique wire-like nanostructures on TiO2 (N) substrates, while formed relatively straightandthickerrod-shapedprecipitatesontheothertwotitaniamaterials. Conclusion/Significance: Our results suggested that proper forms of silver on various titania materials could further influencethebactericidalproperty. Citation: Wong M-S, Sun D-S, Chang H-H (2010) Bactericidal Performance of Visible-Light Responsive Titania Photocatalyst with Silver Nanostructures. PLoS ONE5(4):e10394.doi:10.1371/journal.pone.0010394 Editor:StefanBereswill,Charite′-Univer