N-Type Thermoelectric Performance of Functionalized Carbon Nanotube-Filled Polymer Composites 英文参考文献.docVIP

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N-Type Thermoelectric Performance of Functionalized Carbon Nanotube-Filled Polymer Composites 英文参考文献.doc

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N-Type Thermoelectric Performance of Functionalized Carbon Nanotube-Filled Polymer Composites 英文参考文献

N-TypeThermoelectricPerformanceofFunctionalized CarbonNanotube-FilledPolymerComposites DallasD.Freeman,KyungwhoChoi,ChoonghoYu* DepartmentofMechanicalEngineering,TexasAMUniversity,CollegeStation,Texas,UnitedStatesofAmerica Abstract Carbon nanotubes (CNTs) were functionalized with polyethyleneimine (PEI) and made into composites with polyvinyl acetate (PVAc).CNTs weredispersed withdifferent amountsofsodiumdodecylbenzenesulfonate (SDBS) priortothePEI functionalization. The resulting samples exhibit air-stable n-type characteristics with electrical conductivities as great as 1500S/m andthermopowers as large as 2100mV/K. Electrical conductivity andthermopower werestrongly affected by CNT dispersion, improving the properties with better dispersion with high concentrations of SDBS. This improvement is believedtobeduetotheincreaseinthenumberoftubesthatareevenlycoatedwithPEIinabetter-dispersedsample. Increasing the amount of PEI relative to the other constituents positively affects thermopower but not conductivity. Air exposurereducesboththermopowerandconductivitypresumablyduetooxygendoping(whichmakesCNTsp-type),but stablevalueswerereachedwithinsevendaysfollowingsamplefabrication. Citation:FreemanDD,ChoiK,YuC(2012)N-TypeThermoelectricPerformanceofFunctionalizedCarbonNanotube-FilledPolymerComposites.PLoSONE7(11): e47822.doi:10.1371/journal.pone.0047822 Editor:AristidesDocoslis,Queen’sUniversityatKingston,Canada ReceivedApril30,2012;AcceptedSeptember17,2012;PublishedNovember2,2012 Copyright: ? 2012 Freeman et al. This is an open-access article distributed under the terms of the Creative Commons Attribution License, which permits unrestricteduse,distribution,andreproductioninanymedium,providedtheoriginalauthorandsourcearecredited. Funding:TheauthorsgratefullyacknowledgefinancialsupportsfromtheUSAirForceOfficeofScientificResearch(FA9550-09-1-0609)undertheauspicesofDr. CharlesLee,II-VIfoundation,andthePioneerResearchCenterProgramthroughtheNationalResearchFoundationofKorea(201