原创力文档comparison of the biological properties of several marine sponge-derived sesquiterpenoid quinones比较几种海洋生物属性的sponge-derived sesquiterpenoid醌类.pdfVIP
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comparison of the biological properties of several marine sponge-derived sesquiterpenoid quinones比较几种海洋生物属性的sponge-derived sesquiterpenoid醌类
Molecules 2007, 12, 1376-1388
molecules
ISSN 1420-3049
© 2007 by MDPI
/molecules
Full Paper
Comparison of the Biological Properties of Several Marine
Sponge-Derived Sesquiterpenoid Quinones
Cherie A. Motti 1,*, Marie-Lise Bourguet-Kondracki 2,†, Arlette Longeon 2, Jason R. Doyle 1,
Lyndon E. Llewellyn 1, Dianne M. Tapiolas 1 and Ping Yin 3,‡
1 Australian Institute of Marine Science, Townsville, Queensland, 4810, Australia
2 Laboratoire de Chimie et Biochimie des Substances Naturelles, Muséum National d’Histoire
Naturelle, 57 rue Cuvier (CP 54), Paris, 75005, France ; †E-mail: bourguet@mnhn.fr
3 Nufarm Australia Limited, Department of Chemistry, Macquarie University, North Ryde, NSW,
2109, Australia; ‡E-mail: ping.yin@.au
* Author to whom correspondence should be addressed; Tel: + 61-7-4753 4143; Fax: + 61-7-4772
5852; E-mail: c.motti@.au
Received: 18 June 2007; in revised form: 6 July 2007 / Accepted: 9 July 2007 / Published: 11 July
2007
Abstract: Eight naturally occurring marine-sponge derived sesquiterpenoid quinones were
evaluated as potential inhibitors of pyruvate phosphate dikinase (PPDK), a C4 plant
regulatory enzyme. Of these, the hydroxyquinones ilimaquinone, ethylsmenoquinone and
smenoquinone inhibited PPDK activity with IC50 ’s (reported with 95% confidence
intervals) of 285.4 (256.4 – 317.7), 316.2 (279.2 – 358.1) and 556.0 (505.9 – 611.0) μM,
respectively, as well as being phytotoxic to the C4 plant Digitaria ciliaris . The potential
anti-inflammatory activity of these
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