on the electrooxidation and amperometric detection of no gas at the ptnafion？ electrode没有气体的电氧化和测量电流的检测ptnafion 电极.pdfVIP

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on the electrooxidation and amperometric detection of no gas at the ptnafion？ electrode没有气体的电氧化和测量电流的检测ptnafion 电极.pdf

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on the electrooxidation and amperometric detection of no gas at the ptnafion？ electrode没有气体的电氧化和测量电流的检测ptnafion 电极

Sensors 2003, 3, 290–303 sensors ISSN 1424-8220 2003 by MDPI /sensors On the Electrooxidation and Amperometric Detection of NO Gas at the Pt/Nafion Electrode Kuo-Chuan Ho*, Wen-Tung Hung and Jin-Cherng Yang Department of Chemical Engineering, National Taiwan University, Taipei, Taiwan 10617, R. O. C. Tel. (+886) 2-2366-0739, Fax (+886) 2-2362-3040, e-mail: kcho @.tw * Author to whom correspondence should be addressed. Received: 22 May 2003 / A ccep ted: 03 June 2003 / Published: 22 A ugust 2003 Abstract: The electrochemical oxidation of nitric oxide (NO) gas at the Pt/Nafion electrode has been studied at a concentration of 500 ppm. The electrooxidation of NO taking place over a wide potential range can be described by a transcendental equation, from which the half-wave potential of the reaction can be determined. For NO oxidation with appreciable overpotentials but negligible mass-transfer effects, the Tafel kinetics applies. The obtained charge transfer coefficient () and the exchange current density (i ) are 0.77 o 2 and 14 A/cm , respectively. An amperometric NO gas sensor based on the Pt/Nafion electrode has been fabricated and tested over the NO concentration range from 0 to 500 ppm.