原创力文档recent advances in the application of selectfluortmf-teda-bf4 as a versatile mediator or catalyst in organic synthesis应用的最新进展selectfluortmf-teda-bf4多才多艺的中介或催化剂在有机合成.pdfVIP
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recent advances in the application of selectfluortmf-teda-bf4 as a versatile mediator or catalyst in organic synthesis应用的最新进展selectfluortmf-teda-bf4多才多艺的中介或催化剂在有机合成
Molecules 2011, 16, 6432-6464; doi:10.3390/molecule
OPEN ACCESS
molecules
ISSN 1420-3049
/journal/molecules
Review
Recent Advances in the Application of SelectfluorTMF-TEDA-BF4
as a Versatile Mediator or Catalyst in Organic Synthesis
Stojan Stavber 1,2
1 Laboratory for Organic and Bioorganic Chemistry, “Jožef Stefan” Institute, Jamova 39,
1000 Ljubljana, Slovenia
2 Centre of Excellence CIPKeBiP, Jamova 39, 1000 Ljubljana, Slovenia;
E-Mail: stojan.stavber@ijs.si; Tel.: +386-1-477-3660, Fax: +386-1-423-5400
Received: 14 June 2011; in revised form: 5 July 2011 / Accepted: 19 July 2011 /
Published: 29 July 2011
Abstract: SelectfluorTM F-TEDA-BF4 (1-chloromethyl-4-fluoro-1,4-diazoniabicyclo
[2.2.2]octane bis(tetrafluoroborate) is not only one of the most efficient and popular
reagents for electrophilic fluorination, but as a strong oxidant is also a convenient mediator
or catalyst of several “fluorine-free” functionalizations of organic compounds. Its
applications as a mediator in transformations of oxidizable functional groups or
gold-catalyzed C-C and C-heteroatom oxidative coupling reactions, a catalyst in formation
of various heterocyclic rings, a reagent or catalyst of various functionalizations of
electron-rich organic compounds (iodination, bromination, chlorination, nitration,
thiocyanation, sulfenylation, alkylation, alkoxylation), a catalyst of one-pot-multi-
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