reversible thermochromic nanocomposites based on thiolate-capped silver nanoparticles embedded in amorphous polystyrene可逆热变色基于thiolate-capped银纳米粒子嵌入到非晶态聚苯乙烯纳米复合材料.pdfVIP

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reversible thermochromic nanocomposites based on thiolate-capped silver nanoparticles embedded in amorphous polystyrene可逆热变色基于thiolate-capped银纳米粒子嵌入到非晶态聚苯乙烯纳米复合材料.pdf

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reversible thermochromic nanocomposites based on thiolate-capped silver nanoparticles embedded in amorphous polystyrene可逆热变色基于thiolate-capped银纳米粒子嵌入到非晶态聚苯乙烯纳米复合材料

Materials 2009, 2, 1323-1340; doi:10.3390/ma2031323 OPEN ACCESS materials ISSN 1996-1944 /journal/materials Review Reversible Thermochromic Nanocomposites Based on Thiolate-Capped Silver Nanoparticles Embedded in Amorphous Polystyrene Gianfranco Carotenuto 1,* and Francesca Nicolais 2 1 Institute of Composite and Biomedical Materials, National Research Council, Piazzale Tecchio, 80 – 80125 Napoli, Italy 2 Department of Communication Sciences, University of Salerno, Via Ponte don Melillo – 84084 Fisciano, Salerno, Italy; E-Mail: franicolais@ (F.N.) * Author to whom correspondence should be addressed; E-Mail: giancaro@unina.it; Tel. (+39) 081 7758833; Fax: (+39) 081 7758850. Received: 30 August 2009; in revised form: 15 September 2009 / Accepted: 16 September 2009 / Published: 18 September 2009 Abstract: Technologically useful reversible thermochromic materials can be prepared using very simple polymer-embedded nanostructures. In particular, silver nanoparticles capped by long-chain alkyl-thiolate molecules (i.e., Ag (SC H ) , with n 10) x n 2n+1 y spontaneously organize in aggregates because of the interdigitation phenomenon involving the linear alkyl chains bonded at surfaces of neighboring nanoparticles. Owing to the alkyl- chain interdigitation, nanoparticles very close to each other result and an interaction among their surface plasmon resonances may take place