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Comparison of Two Source Apportionment Models OASIS Abstract 两个源解析模型比较抽的绿洲.doc

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Comparison of Two Source Apportionment Models OASIS Abstract 两个源解析模型比较抽的绿洲

Comparison of Two Source Apportionment Models for Fine Particulate Matter In Chicago, Illinois Michael Rizzoa and Peter Scheffb aUnited States Environmental Protection Agency, 77 W. Jackson Blvd., Chicago, IL 60604 bUniversity of Illinois – Chicago, School of Public Health, 2121 W. Taylor St., Chicago, IL 60612 INTRODUCTION In 2000, the United States Environmental Protection Agency established the Fine Particulate Speciation Trends Network to expand on its existing PM2.5 monitoring activities. The purpose of the network is to characterize individual species which compose the total fine particulate measured at the Agencys Federal Reference Method (FRM) PM2.5 monitoring sites. The data from the speciation network serves an important role in aiding the Agency in determining which species are the most prevalent in areas of the nation thus allowing for the formulation of control strategies. Studies have already shown that secondary sulfates comprise a large part of the fine particulate in the Eastern part of the United States while secondary nitrates dominate the total PM2.5 in the Western United States. The Midwestern section of the country is dominated by both secondary sulfates and nitrates. All areas of the country have been shown to have a large portion of the total fine particulate comprised of organic carbon.1 Another use which has been planned for the data collected through the speciation network is to determine possible fine particulate sources. Traditional source apportionment techniques have centered around the use of the chemical mass balance model which utilizes source profiles and speciated data to determine source contributions for either gaseous or particulate compounds or a combination of both.2,3,4 There have been many analyses conducted regarding volatile organic compounds.5,6,7,8,9,10,11 Recently, more studies have focused on implementing the chemical mass balance technique for fine particulate matter. However, source profiles for many of the