生物阴极微生物燃料电池处理垃圾渗滤液及产电性能分析-treatment of landfill leachate by bio-cathode microbial fuel cell and analysis of its electricity production performance.docxVIP

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生物阴极微生物燃料电池处理垃圾渗滤液及产电性能分析-treatment of landfill leachate by bio-cathode microbial fuel cell and analysis of its electricity production performance.docx

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生物阴极微生物燃料电池处理垃圾渗滤液及产电性能分析-treatment of landfill leachate by bio-cathode microbial fuel cell and analysis of its electricity production performance

重庆大学重庆大学硕士学位论文中文摘要 II II 为曝气MFC不曝气MFC化学MFC。结果表明，曝气MFC更利于渗滤液中N的去除。另外，阴极缓冲液对MFC处理垃圾渗滤液液有一定影响，其中扩散至阳极的 TP随渗滤液浓度的升高而减小，且低于阴极TP的去除量；各组MFCs的阳极出水中 TP均维持在一定的浓度范围，依次为曝气MFC(16.55mg/L)不曝气MFC (19.13 mg/L)化学MFC (23.65mg/L)。化学 MFC 和曝气 MFC 利用 100%的垃圾渗滤液进行产电时，最大输出电压分别为 698.9715mV、459.4029mV，最大输出功率为 197.73 mW/m3、147.65 mW/m3，内阻均上升分别为 900Ω、700Ω；经过 45d 运行产电后，COD 由初始的 6332.11mg/L 分别降至 2752.41mg/L、2261.72mg/L，去除率分别为 56.53%、64.28%，库伦效率分别为 14.28%、17.10%；氨氮的去除比例分别为 53.78%、58.09%，均出现了阳极室中高浓度的 NH4+通过质子交换膜扩散到阴极的现象。关键词：微生物燃料电池，生物阴极，垃圾渗滤液，污染物降解，产电特性重庆大学重庆大学硕士学位论文英文摘要 III III ABSTRACT Landfill leachate shows characteristics of high colority, big stink, high toxicity and difficult to handle due to higher COD, BOD, NH3-N, heavy metal ions and toxic organic pollutants. Because of bad smell, high toxicity and difficult treatment the lechate has serious harmer to the environment. From the removal of contaminants and producing electricity, the advantages of biological cathode type microbial fuel cell (MFC) are easily building, low operating cost, avoiding the secondary pollution and removing the nitrogen by denitrification reaction. Using potassium ferricyanide as dual chamber chemical-cathode MFC cathode electron acceptor for reference, the double chamber aeration-cathode MFC and noaeration-cathode MFC were built to track and compare their startup conditions and performance. The electricity production and degradation effect of pollutants were explored by disposing landfill leachate with using different type cathode MFCs. The startup of MFC is essentially the process that the electricity producing microorganism enrichs and forms biofilm gradually in anode surface. Under the condition of NaAC anode carbon source, the startup time was in order: chemical MFC (1d) aeration MFC(5d) noaeration MFC (10d). The stable cycle order was following as, noaeration MFC(30d) aeration MFC(25d) chemical MFC(20d). The order of stab- le voltage of electricity production was aeration MFC(618mV) noaeration MFC