石墨烯基光催化剂的制备及其对甲基橙光催化降解的分析-preparation of graphene-based photocatalyst and analysis of photocatalytic degradation of methyl orange.docxVIP

AbstractInmodernsociety,theprocessofindustrializationmismanagedhascausedaglobalenvironmentalpollutionandecologicaldestruction,resultedinaffectinghumansurvivalanddevelopment.Photocatalystplaysauniqueroleforitsenvironmentallyfriendlyfeaturesinthefieldofenvironmentalprotection.Sofar,photocatalyststudieshavebeenmadeagreatprogress.Buttherearestillmanyneedstobefurtherstudied.Thispaperwasfocusedonthetraditionalphotocatalystforitselectron-holepairseasilyregenerated,causingphotocatalyticeffiency.Soweusegrapheneasa2DphotocatalysttoimprovethephotocatalyticpropertiesofVis-light.ThispaperwaspreparedtotakeHummersmethodtoobtaingraphiteoxide.Andthenweobtainthegrapheneoxidewiththeultrasonictreatmentinwater.WeuseFT-IR、Raman、XPS、SEM、TEM、AFM、UV-vimeanstoanalysisitssurfacestructure,morphology,bondingelementandcharacterization.TheresultsshowthatthesurfaceofGOcontainsalargenumberofcontaininggrouponthesurfaceofgraphene.Inthispaperweusethesitusol-gelmethodtoobtainGO-TiO2.Asa2DvectorofTiO2,wefoundthatthecrystalformofTiO2haven’tbeenchangedaftercomplexed.ThispaperstudiedmanyfactorsaffectingthedegradationofMOWithGO-TiO2catalyst,forexample,thecontantofGO-TiO2,thepHofsolutionandsoon.WefoundthatwhenthepHwas4.0andthecontantoftheGO-TiO2was300mg/L,thedegradationrateofMOcanreachupto32.719%.InthispaperweusesituhomogeneousprecipitationmethodtoobtainGO-ZnO.WeuseionexchangedmethodtoimprovetherecombinationratebetweenGOandZnO.Asa2DvectorofZnO,withoutchangingthecrystalformaftercomplexed.ThispaperstudiedmanyfactorsaffectingthedegradationofMOWithGO-ZnOcatalyst,forexample,thecalcinationtemperatureofGO-ZnO,thepHofsolutionandsoon.WefoundthatwhenthepHwas4.0andthecontantoftheGO-ZnOwas300mg/L,thedegradationrateofMOcanreachupto22.312%.ConsideringthepoorsolubilityofC60asaphotocatalyst,weproposetousetheaminoacidtomodifyit.Sothatincreasingitsdegreeofgraphenebasedoxidecomposite.ThroughFT-IR、Raman、XPS、TEMmeanstoanalysisitssurfacestructure,bondingelement,characterizationandcrystalstructure.Theresultsshowthatthesurfaceofmod