活性炭混合填料对低温等离子体去除含甲苯废气性能影响的试验分析-环境工程专业论文.docxVIP

西安建筑科技大学硕士学位论文 西安建筑科技大学硕士学位论文 西安建筑科技大学硕士学位论文 西安建筑科技大学硕士学位论文 Experimental Study on Effects of Activated Carbon Mixed Filler on Decontamination of Toluene-containing Exhaust Gas Using Non-thermal Plasma Specialty: Environment Engineering Name: Zhang Qing Instructor: Dang Xiaoqing Abstract This paper used toluene-containing exhaust gas as the experimental object, used the activated carbons and ceramic rings filler which mixed in a certain proportion, to research how the packed bed reactor impacts toluene removal performance. Ceramic rings in the mixed filler could be conducive to enhancing the intensity of discharge, and activated carbons could improve the adsorption capacity of fillers. Thus further reduced the energy consumption of the reactor, and reduced or avoided secondary pollution.This paper also did some systematic research on plasma regeneration of the activated carbon in the mixed filler. The main results were as follows: According to the voltage-current wave forms, the mixed filler increased the number of reactor’s micro discharge, reduced the maximum amplitude of pulse current, so that the discharge became more uniform and stable; but also can effectively inhibited the gas breakdown. Compared to single mixed filler adsorption of toluene, the breakthrough time of adsorption can be extended for 75min. The toluene removal rate increased more obviously（18.9%） when the filler mixing ratio raised from 1:24 to 1:12, but only increased 1.1% when the filler mixing ratio raised from 1:12 to 1:8. The toluene removal rate increased significantly with enhancing of applied voltage, while decreased with increasing of empty tower gas velocity and inlet concentration. During toluene degradation process, only detected CO, CO2, H2O and a small amount of O3 from outlet of reactor. According to the analysis of FT-IR and GC/MS, the intermediate product of the degradation of toluene which adsorbed by activated carbon were benzaldehyde, benzoic acid, benzene and ethers. This i