磷钨酸氧化石墨烯复合材料的制备及其催化性能的研究-工业催化专业论文.docxVIP

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磷钨酸氧化石墨烯复合材料的制备及其催化性能的研究-工业催化专业论文.docx

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PAGE PAGE IV ABSTRACT MO by O2?-and ?OH plays a major role in the photocatalytic degradation process. 3. The catalytic oxidative desulfurization of model oil with PW12/GO-NH2 is performed in the presence of H2O2 oxidant. The effects of temperature, the dose of catalysts, H2O2/DBT molar ratio and solvents were investigated in detail. It reveals that, PW12/GO-NH2 exhibit the best catalytic activity compared with PW12, GO-NH2 as well as the mixture of them, the sulfur removal in n-octane phase can reach to 100% when react 2 h with the temperature of 60 oC. The efficiency for the removal of DBT is still preserved with 90% after four cycles. Key Words: Polyoxometalates; Graphene oxide; Adsorption; Photocatalysis; Desulfurization 目目录目录第 1 章绪论 ············································································································ 1 1.1 前言·············································································································· 1 1.2 多聚金属含氧酸概述 ·················································································· 2 1.2.1 多聚金属含氧酸简介········································································ 2 1.2.2 磷钨酸简介 ······················································································· 4 1.3 氧化石墨烯简介 ·························································································· 9 1.3.1 氧化石墨烯 ······················································································· 9 1.3.2 氧化石墨烯的性质 ········································································· 10 1.3.3 氧化石墨烯的应用 ········································································· 11 1.4 选题目的、意义及研究内容····································································· 15 1.4.1 选题目的及意义 ············································································· 15 1.4.2 研究内容 ························································································· 1