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离子液体在混合溶液聚集.pdf

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Journal of Molecular Liquids 130 (2007) 104 – 107 /locate/molliq Aggregates in mixtures of ionic liquids Stefan Thomaier, Werner Kunz ⁎ Institute of Physical and Theoretical Chemistry, University of Regensburg, D-93040, Germany Received 15 March 2006; accepted 25 April 2006 Available online 28 July 2006 Abstract Surfactant-like ionic liquids (C MIMCl, C MIMBF ) aggregate in mixtures with another ionic liquid (EAN). Critical aggregate concen- 16 16 4 trations and estimations of object sizes are given and compared to aqueous systems and other relevant literature data. The investigated mixtures are stable up to more than 200 °C and can probably be used to extend the limited temperature range of water-based colloids. © 2006 Elsevier B.V. All rights reserved. Keywords: Ionic liquids; Micelles; Colloids 1. Introduction lamellar liquid-crystal phases in EAN was reported over twenty years ago [22–24]. Over the last years the interest in ionic liquids (IL) has in- Based on these preceding papers, we studied a colloidal sys- creased rapidly because of their unique properties [1] They have tem, which is based on a mixture of two ionic liquids. Although shown to be applicable as solvents in organic reactions or catalysis preceding studies with pyridinium salts as surfactants gave rise to [2] a