Visible-Light Photocatalytic Activity and Deactivation Mechanism of Ag3PO4 Spherical Particles外文翻译.pdfVIP

FULL PAPER DOI: 10.1002/asia.201200197 Visible-Light Photocatalytic Activity and Deactivation Mechanism of Ag3PO4 Spherical Particles Wenguang Wang,[a] Bei Cheng,[a] Jiaguo Yu,*[a] Gang Liu,*[b] and Wenhong Fan*[c] Abstract: Ag PO spherical particles ning electron microscopy (SEM), and our mechanism, Ag nanoparticles de- 3 4 were synthesized by a facile precipita- transmission electron microscopy posited on Ag3PO4 acted as electron tion method using silver nitrate and (TEM), a possible mechanism responsi- trapping centers to prevent photogen- Na2HPO4 as precursors. The as-pre- ble for the improvement and subse- erated electron-hole pairs from recom- pared samples had a high photocatalyt- quent decline of the photocatalytic per- bination. A further increase in the re- ic activity toward Rhodamine B (RhB) formance of Ag3PO4 is proposed. cycle times decreases the photocatalyt- degradation under visible-light illumi- Ag3PO4 spherical particles recycled for ic activity owing to the shielding effect nation. With increasing recycling times four times showed the highest photoca- by Ag layers on the surface of Ag PO . 3 4 the photocatalytic activity first in- talytic activity because, according to The results presented herein shed new creased and then decreased. Based on lig