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c e o c比p q s佐治亚技术研究所（ o c e c ratio p a q s- georgia instituteof technology）.doc

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c e o c比p q s佐治亚技术研究所（ o c e c ratio p a q s- georgia instituteof technology）

Estimating the secondary organic aerosol contribution to PM2.5 using the EC tracer method. Juan C. Cabada and Spyros N. Pandis, Department of Chemical Engineering, Carnegie Mellon University, 5000 Forbes Ave., Pittsburgh, PA 15213 Ramachandran Subramanian and Allen L. Robinson, Department of Mechanical Engineering, Carnegie Mellon University, 5000 Forbes Ave., Pittsburgh, PA 15213 Andrea Polidori and Barbara Turpin, Department of Environmental Sciences, Rutgers University, 14 College Farm Road, New Brunswick, NJ 08901 Abstract The EC tracer method is applied to a series of measurements by different carbonaceous aerosol samplers in the Pittsburgh Air Quality Study (PAQS) in order to estimate the concentration of secondary organic aerosol. High-resolution measurements (2-6 hrs) and daily averaged concentrations were collected during the summer 2001 intensive (July 1 to August 4, 2001) and are used for the analysis. The various samplers used during PAQS show differences in the measured concentrations of OC and EC due to the different sampling artifacts and sampling periods. A systematic approach for the separation of periods where SOA contributes significantly to the ambient OC levels from the periods where organic and elemental carbon concentrations are dominated by primary emissions is proposed. Ozone is used as indicator of photochemical activity to identify periods of probable secondary organic aerosol production in the area. Gaseous tracers of combustion sources (CO, NO, and NOx) are used to identify periods where most of the OC is primary. Periods dominated by primary emissions are used to establish the relationship between primary OC and EC, a tracer for primary combustion-generated carbon for the different sets of measurements for July 2001. Around 35% of the organic carbon concentration in Western Pennsylvania during July of 2001 is estimated to be secondary in origin. 1. Introduction Carbonaceous aerosol is an important constituent of the PM2.5 (particulate