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The importance of back contact modification in Cu2ZnSnSe4 solar cells The role of a thin MoO2 layer.pdf

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The importance of back contact modification in Cu2ZnSnSe4 solar cells The role of a thin MoO2 layer.pdf

Nano Energy 26 (2016) 708–721Contents lists available at ScienceDirectNano Energyhttp://d 2211-28 n Corr E-m 1 Pr na, Austjournal homepage: /locate/nanoenThe importance of back contact modification in Cu2ZnSnSe4 solar cells: The role of a thin MoO2 layer S. Lopez-Marino a,n,1, M. Espíndola-Rodríguez a, Y. Sánchez a, X. Alcobé b, F. Oliva a, H. Xie a, M. Neuschitzer a, S. Giraldo a, M. Placidi a, R. Caballero c, V. Izquierdo-Roca a, A. Pérez-Rodríguez a,d, E. Saucedo a a Catalonia Institute for Energy Research (IREC), Jardin de les Dones de Negre 1, 08930 Sant Adrià del Besòs, Spain b Centres Científics i Tecnològics de la Universitat de Barcelona (CCiTUB), LLuís Solé i Sabarís 1-3, 08028 Barcelona, Spain c Universidad Autónoma de Madrid, Applied Physics Department, Francisco Tomás y Valiente 7, 28049 Madrid, Spain d Departament de Electrònica (IN2UB), Universitat de Barcelona, Martí i Franquès 1, 08028 Barcelona, Spaina r t i c l e i n f o Article history: Received 9 September 2015 Received in revised form 1 June 2016 Accepted 18 June 2016 Available online 23 June 2016 Keywords: Cu2ZnSnSe4 MoO2 MoSe2 Solar cells Back /10.1016/j.nanoen.2016.06.034 55/ 2016 Elsevier Ltd. All rights reserved. esponding author. ail address: simonlopez_iq@ (S. L esent address: Crystalsol GmbH, Simmeringe ria.a b s t r a c t Cu2ZnSn(SxSe1x)4 (CZTSSe) photovoltaic absorbers could be the earth-abundant and low toxicity re- placement for the already commercialized CuIn1xGaxSe2 (CIGS) thin film technology. In order to make this possible, specific research efforts applied to the bulk, front and back interfaces must be performed with the aim of improving CZTSSe performance. In this paper the importance of back contact mod- ification to obtain high efficiency Cu2ZnSnSe4 (CZTSe) solar cells and to increase a paramount and lim- iting parameter such as VOC is highlighted. Several Mo configurations (monolayer, bi-layer and tri-layer) with different electrical and morphological properties are inves