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Thermodynamic analysis of effects of contact angle on interfacial interactions and its implications for membrane fouling control.pdf

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Thermodynamic analysis of effects of contact angle on interfacial interactions and its implications for membrane fouling control.pdf

Bioresource Technology 201 (2016) 245–252 Contents lists available at ScienceDirect Bioresource Technology journal homepage: /locate/biortech Thermodynamic analysis of effects of contact angle on interfacial interactions and its implications for membrane fouling control Jianrong Chen a, Liguo Shen a, Meijia Zhang a, Huachang Hong a, Yiming He b, Bao-Qiang Liao c, Hongjun Lin a,? a College of Geography and Environmental Sciences, Zhejiang Normal University, Jinhua 321004, PR China b Department of Materials Physics, Zhejiang Normal University, Jinhua 321004, PR China c Department of Chemical Engineering, Lakehead University, 955 Oliver Road, Thunder Bay, Ontario P7B 5E1, Canada highlights Total interaction energy monotonically decreases with water contact angle. Total interaction energy monotonically increases with glycerol contact angle. Water and glycerol contact angle are reliable indicators predicting interaction. Membrane roughness remarkably decreases interaction strength. Diiodomethane contact angle has minor effect on the total interaction. article info Article history: Received 15 October 2015 Received in revised form 24 November 2015 Accepted 25 November 2015 Available online 28 November 2015 Keywords: Membrane bioreactor Membrane fouling Hydrophilicity Interfacial interaction Contact angle abstract Concept of hydrophobicity always fails to accurately assess the interfacial interaction and membrane fouling, which calls for reliable parameters for this purpose. In this study, effects of contact angle on interfacial interactions related to membrane fouling were investigated based on thermodynamic analysis. It was found that, total interaction energy between sludge foulants and membrane monotonically decreases and increases with water and glycerol contact angle, respectively, indicating that these two parameters can be reliable indicators predicting total interaction energy and membrane fouling. Membrane roughness decreases interaction strength for ov