Angular Dependence of Fluorescence Emission from Quantum Dots inside a Photonic Crystal英文文献资料.docVIP
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Angular Dependence of Fluorescence Emission from Quantum Dots inside a Photonic Crystal英文文献资料
HindawiPublishingCorporation
ResearchLettersinNanotechnology
Volume2008,ArticleID974072,4pages
doi:10.1155/2008/974072
ResearchLetter
AngularDependenceofFluorescenceEmissionfrom
QuantumDotsinsideaPhotonicCrystal
KasperBaert,1BrankoKolaric,1WimLibaers,1RenaudA.L.Valle′e,1MarcelDiVece,2
PeterLievens,2andKoenClays1
1
DepartmentofChemistry,InstituteofNanoscalePhysicsandChemistry(INPAC),KatholiekeUniversiteitLeuven,
Celestijnenlaan200D,3001Heverlee,Belgium
2
LaboratoryofSolidStatePhysicsandMagnetism,InstituteofNanoscalePhysicsandChemistry(INPAC),
KatholiekeUniversiteitLeuven,Celestijnenlaan200D,3001Heverlee,Belgium
CorrespondenceshouldbeaddressedtoKoenClays,koen.clays@fys.kuleuven.be
Received23January2008;Accepted2April2008
RecommendedbyJe?eryL.Co?er
The?uorescenceofemittersembeddedinaphotoniccrystalisknowntobeinhibitedbythepresenceofanincompletephotonic
bandgaporpseudogapactingintheiremissionrange.Here,wepresentastudyoftheangulardependenceofthe?uorescence
emissionofemittersembeddedinaphotoniccrystal.Ourresultsclearlyshowanangulardependenceofthe?uorescenceemission,
whichiscausedbythepresenceofanincomplete3Dbandgap.
Copyright?2008KasperBaertetal.ThisisanopenaccessarticledistributedundertheCreativeCommonsAttributionLicense,
whichpermitsunrestricteduse,distribution,andreproductioninanymedium,providedtheoriginalworkisproperlycited.
1.
INTRODUCTION
the refractive index of the colloidal spheres determine the
spectralpositionofthebandgap.Thecombinationofthese
densecrystalstructures(fccorRhcp)withthelow-refractive
index of most monodisperse spherical colloidal particles
(latex,silica)resultsinanincompletebandgap(pseudogap
orstopband)[7],thatis,agapwithpropertiesdependingon
theincidenceangleoftheimpinginglight.Inthisstudy,we
presenttheangulardependenceofthe?uorescenceemission
ofemittersembeddedinPCs.Ourinvestigationsshowthat
theangulardependenceofthepseudogapcausesashiftin
boththemaximumof?uorescenceintensityaswellasinthe
reducedemissionoftheembeddedemitters.These?ndings
canbeu
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