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Asymmetric Composite Nanoparticles with Anisotropic Surface Functionalities英文文献资料.doc

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Asymmetric Composite Nanoparticles with Anisotropic Surface Functionalities英文文献资料

HindawiPublishingCorporation JournalofNanomaterials Volume2009,ArticleID620269,5pages doi:10.1155/2009/620269 ResearchArticle AsymmetricCompositeNanoparticleswith AnisotropicSurfaceFunctionalities YilongWang, HongXu, WeiliQiang, HongchenGu, 1 1 1 1andDongluShi 2,3 1 2 3 NanoBiomedicineResearchCenter,Med-XResearchInstitute,ShanghaiJiaoTongUniversity,Shanghai200030,China DepartmentofChemicalandMaterialsEngineering,UniversityofCincinnati,Cincinnati,OH45221,USA NationalKeyLaboratoryofNano/MicroFabricationTechnology,ResearchInstituteforMicro/NanoScienceandTechnology, ShanghaiJiaoTongUniversity,Shanghai200030,China CorrespondenceshouldbeaddressedtoHongchenGu,hcgu@ Received28June2008;Accepted17November2008 RecommendedbyJoseA.Pomposo Asymmetric inorganic/organic composite nanoparticles with anisotropic surface functionalities represent a new approach for creatingsmartmaterials,requiringtheselectiveintroductionofchemicalgroupstodualcomponentsofcomposite,respectively. Here,wereportthesynthesisofsnowman-likeasymmetricsilica/polystyreneheterostructurewithanisotropicfunctionalitiesviaa chemicalmethod,creatingnanostructurepossiblyo?eringtwo-sidedbiologicaccessibilitythroughthechemicalgroups.Carboxyl groupwasintroducedtopolystyrenecomponentofthesnowman-likecompositesbyminiemulsionpolymerizationofmonomer on local surface of silica particles. Moreover, amino group was then grafted to remained silica surface through facile surface modi?cationofthecompositenanoparticles.Theasymmetricshapeofthesecompositeswascon?rmedbyTEMcharacterization. Moreover,characteristicsofanisotropicsurfacefunctionalitieswereindicatedbyZetapotentialmeasurementandconfocallaser microscopyafterbeinglabeledwith?uorescentdyes.Thisstructurecould?ndpotentialuseascarriersforbiologicalapplications. Copyright?2009YilongWangetal.ThisisanopenaccessarticledistributedundertheCreativeCommonsAttributionLicense, whichpermitsunrestricteduse,distribution,andreproductioninanymedium,provided