Bridged Phthalocyanine Systems for Sensitization of Nanocrystalline TiO2 Films英文文献资料.docVIP

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Bridged Phthalocyanine Systems for Sensitization of Nanocrystalline TiO2 Films英文文献资料.doc

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Bridged Phthalocyanine Systems for Sensitization of Nanocrystalline TiO2 Films英文文献资料

HindawiPublishingCorporation InternationalJournalofPhotoenergy Volume2010,ArticleID136807,11pages doi:10.1155/2010/136807 ResearchArticle BridgedPhthalocyanineSystemsforSensitizationof NanocrystallineTiO2Films GloriaZanotti, GiovannaPennesi, AldoDiCarlo, AndreaReale, 1 NicolaAngelini, GentilinaRossi, ThomasM.Brown, 2 SaraNotarantonio, AnnaMariaPaoletti, 2 AngeloLembo, DanieleColonna, andGiuseppeCalogero 2 2 2 1 1 1 1 1 3 1 CenterforHybridandOrganicSolarEnergy(CHOSE),UniversityofRome“TorVergata”,ViaGiacomoPeroni400/402, 00131Rome,Italy 2 3 CNR-IstitutoStrutturadellaMateria,ViaSalariaKm.29.5,MonterotondoStazione,00016Rome,Italy CNR,IstitutoperiProcessiChimico-Fisici,SalitaSperoneContradaPapardo,FaroSuperiore,98158Messina,Italy CorrespondenceshouldbeaddressedtoGentilinaRossi,gentilina.rossi@r.it Received1June2010;Accepted28June2010 AcademicEditor:LeonardoPalmisano Copyright?2010GloriaZanottietal.ThisisanopenaccessarticledistributedundertheCreativeCommonsAttributionLicense, whichpermitsunrestricteduse,distribution,andreproductioninanymedium,providedtheoriginalworkisproperlycited. Phthalocyaninesbased-dyesrepresentattractivealternativestotheexpensiveandpollutingpyridylbasedRucomplexesbecauseof theirphotochemicalandthermalstability,theydoshowinfactintenseabsorptionintheUV/blue(Soretband)andthered/near IR(Qband)spectralregionsandappearverypromisingassensitizerdyesforDSSC.Inthiscontributionwereviewthestateofthe artandtherecentprogressintheapplicationofthesematerialsasdyesforDSSCandpresentthreenewdyeswhicharebridged derivativesofIronphthalocyanine.Synthesis,opticalproperties,electrochemicalcharacterizationanddeviceperformancesare discussedwithregardtothedi?erentsubstitutiondegreeofthemacrocycle. 1.Introduction and a photoinert counter electrode (cathode) [3]. In the moststudiedande?cientdevicestodate,lightisadsorbed by a polypyridyl ruthenium-based complex (dye) that is linkedtotitaniumoxidesurfaceviacarboxylatemoieties;the photoanodeisathick(～12μm)?lmofTiO2nanoparticles