东海北部气溶胶特征.pdfVIP

ARTICLE IN PRESS Atmospheric Environment 41 (2007) 7821–7836 /locate/atmosenv Characterization of aerosol over the Northern South China Sea during two cruises in 2003 Xingying Zhanga,b,c, Guoshun Zhuanga,c,, Jinghua Guoc,d, Kedong Yine, Peng Zhangb aDepartment of Environmental Science and Engineering, The Center for Atmospheric Chemistry Study, Fudan University, Shanghai 200433, China bNational Satellite Meteorological Center, China Meteorological Administration, Beijing 100081, China c The Center for Atmospheric Environmental Study, Beijing Normal University, Beijing 100875, China dAnalytical and Testing Center, Beijing Normal University, Beijing 100875, China eSouth China Sea Institute of Oceanology, Chinese Academy of Science, Guangzhou 510301, China Received 29 October 2006; received in revised form 2 May 2007; accepted 9 June 2007 Abstract Atmospheric transport of trace elements has been found to be an important pathway for their input to the ocean. TSP, PM10, and PM2.5 aerosol samples were collected over the Northern South China Sea in two cruises in 2003 to estimate the input of aerosol from continent to the ocean. About 23 elements and 14 soluble ions in aerosol samples were measured. The average mass concentration of TSP in Cruise I in January (78 mg m3) was twice of that in Cruise II in April (37 mg m3). Together with the crustal component, heavy metals from pollution sources over the land (especially from the industry and automobiles in Guangzhou)