乌梁素海沉积物对磷吸附特性的粒度效应研究-水文学及水资源专业论文.docxVIP

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乌梁素海沉积物对磷吸附特性的粒度效应研究-水文学及水资源专业论文.docx

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乌梁素海沉积物对磷吸附特性的粒度效应研究-水文学及水资源专业论文

Effects ofSedimentParticleSizeonPhosphateAdsorption CharacteristicsintheLakeWuliangsuhaiAbstractEntroficationoflakeshasbeenbecomingoneoftheglobalaquaticeco-environment problems.Ithasbeenprovedthatphosphorusis oneofthekeycontaminantscontributing totheentroficationoflakes.Itisdissolvedandadsorbedinboththewaterbodyandthe sedimentanddynamicallytransportinbetween.Itwasreportedthatthetransport processeswere affectedbymanyfactorslikephysical,chemical,hydrogeochemical, mineralogicaletc,amongwhichtheparticlesizeofthesedimentplayanimportantrolein adsorptioncharacteristics ofphosphorus.Togetbetterunderstandingon theeffectsoftheadsorptioncharacteristicsof phosphorusinthelakeWuliangsuhai,thesedimentwassampledandsievedintofour groupswiththeparticlesizes oflessthan63μm,63-125μm,125-250μmandgreatthan 250μmindividually.Labexperimentswerecarriedoutonphosphorusadsorption dynamics.Theresultsshowedthattheadsorptionprocesseswereaffectedsignificantly bytheparticlesize.Thehigheradsorptionratesappearedinthefirst45minforallthe treatments withdifferentparticlesizes.Meanwhile,the rates werevariedwiththeparticle size throughoutthetestperiod,thegreateroftheparticlesizetheloweroftheadsorption rate.Theadsorptionprocessesshowedthebestagreementwithboththesecond-order equationandLangmuirmodelinthehigherconcentrationsolution.Theamountofthe phosphorusadsorptionhadalinerrelationshipwiththeinitialsubstrateconcentrations andthebalancedconcentrations.Thetest resultsalsosuggestedthat thephosphorus adsorptionwasanendothermicreaction,thehigherofthetemperaturethemoreofthe phosphoruswasadsorbed.pHofthesolutionalsoaffectedtheamountofthephosphorus adsorption,whichwasincreasedfromtheacidtothealkalineconditions.Key words：LakeWuliangsuhai,Surfacesediment, Adsorption,ParticlesizeeffectDirected by:Prof.ZHANGShengApplicantforMasterdegree:GAO Min(Hydrologyandwaterresources)(CollegeofWaterResourcesandCivilEngineering，InnerMongoliaAgriculturalUniversity，Huhhot，010018，China)目录1绪论............................................