改性棉纤维重金属离子的吸附性能分析-analysis of adsorption properties of heavy metal ions on modified cotton fiber.docxVIP

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改性棉纤维重金属离子的吸附性能分析-analysis of adsorption properties of heavy metal ions on modified cotton fiber.docx

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改性棉纤维重金属离子的吸附性能分析-analysis of adsorption properties of heavy metal ions on modified cotton fiber

AbstractStudyontheadsorptionpropertyofmodifiedcottonfiberstoheavymetalionsStudyontheadsorptionpropertyofmodifiedcottonfiberstoheavymetalionsAbstractHeavymetalpollutioniscausedbytheheavymetalsortheircompounds.Afteritentersthehumanbodythroughfoodandwater,thiscanoccurstronginteractionwithproteinsandvariousenzymes,makingthemlosetheiractivity;theymayalsoenrichedincertainorgansofthehumanbody,overdosecancauseacutepoisoning,subacutepoisoning,chronicpoisoningandsoon,thiswillhavegreatharmtohumanbodys.Therefore,treatmentofheavymetalpollutionhasattractedpeoplesattention.Thistopictakecottonfibersasacarrier,successfullypreparedtwomodifiedcottonfiberadsorbentbygraftedtetraethylenepentaminemonomerandHBP-NH2tooxidizedcottonfibers,atthesametimeweoptimizeditspreparationprocess.Themorphologyandstructureofmodifiedcottonfiberwereanalyzedbyscanningelectronmicroscopy(SEM)andinfraredspectroscopy(FT-IR).Theresultsshowedthat:Aftermodified,thelongitudinalstripesinthesurfaceofpretreatedcottonfiberdisappeared;therecontainingalargenumberofaminoandhydroxylactivesitesonthepreparedadsorbentsmolecules,theycanadsorbeandremoveheavymetalsbyChelatingligandswithheavymetalsions.TheadsorptionofHBP-NH2modifiedcottonfiberadsorbentisbetterthantetraethylenepentaminemonomermodifiedcottonfiberadsorbent.ThemaximumadsorptionofPb2+,Cd2+,Cu2+byHBP-NH2modifiedcottonfiberadsorbentcanreached41.38mg/g,28.91mg/g,19.16mg/g.Thispaperdiscussestheinfluenceoftheadsorbentdosage,pH,adsorptionoftime,initialconcentrationofmetalandotherconditionsontheadsorptioneffect.Tohaveabetterunderstandingoftheadsorptionbehaviorforheavymetalions,weuseadsorptionkineticsandadsorptionisothermstofittheexperimentaldataandthenanalysis.Kineticexperimentsshowedthat:Quasi-twoequationsismoresuitabletodescribetheadsorptionprocess,andtheadsorbentshaveahigheradsorptionrateofthethreemetalions,theycanachieveadsorptionequilibriumwithin2h.Adsorptionisothermresultsindicatethat:Langmuirisbestsuitedtodescribetheadsorptionprocessforheavymetalions,whichismonolayerSt