烧结矿烧结过程中so2和nox生成的影响因素分析-analysis of influencing factors of so2 and nox formation in sintering process of sinter.docx

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烧结矿烧结过程中so2和nox生成的影响因素分析-analysis of influencing factors of so2 and nox formation in sintering process of sinter.docx

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烧结矿烧结过程中so2和nox生成的影响因素分析-analysis of influencing factors of so2 and nox formation in sintering process of sinter

AbstractAsweknown,SO2andNOxarethemainairpollutants.Theirtotalemissionsfromthesinteringprocessoccupys40%to60%oftheentiresteelindustryemissions.StudyingtheinfluencefactorsofSO2andNOxformationintheoresinteringprocesshasimportanttheoreticalandpracticalsignificancetoourunderstandingofSO2andNOxproducingapproaches,migrationlawandhowtoreduceemissions.Thisthesisexperimentallyinvestigatedtheeffectsofairflow,moisturecontent,fuelcontentandmixurealkalinityonSO2andNOxreleaseinthesinteringprocess.ThepreliminaryanalysisofSO2andNOxformationmechanismwasalsoconducted.Theresearchcontentandresultsareasfollows:TheairflowhassomedilutioneffectonSO2andNOxconcentrationinsinteringfluegas,buttheincreaseofairflowcanpromotethereleaseofNOx.ThemoisturecontentofthemixturedoesnotsignificantlyimpacttheSO2andNOxconcentration,whileitgreatlyaffectsNO2content.IncreasingthecokecontentofthemixuremakesthetemperatureswhicharecorrespondingtotheSO2andNOxconcentrationpeaksdrop,onthecontrary,thepeakconcentrationrises.ThemixurealkalinityinhibitstheSO2,NOxrelease.Withtheincreasingofalkalinity,theSO2andNOxconcentrationsinfluegashavebeenreduced.Thedifferentsulfuroccurrenceformsresultsinthedifferentreleasingdifficulty.Whenthetemperatureisbetween300℃and500℃,thereexistsSO2releasing.Bythistime,allthesulfurreleasingisfromtheelementalsulfurandorganicsulfurinthesinteringfuel.ThesulfurinFeS2,ZnSandPbScomestoreleasebetween500℃and700℃.Howeverwhenthetemperatureincresesfrom700℃to1000℃,thesulfurinCuFeS2andCu2Sbeginstorelease.NOxinsinteringfluegascanbedividedintothermaltype,prompttypeandfueltype.TemperatureisthemostimportantfactoraffectingtherateofthermalNOxgeneration.Intheactualsinteringprocess,thesinteringtemperatureislowerthanthethermalNOxformationtemperature,sothermalNOxcontentisextremelylowinsinteringfluegas.ThemassofnitrogenelementinNOxisclosetothenitrogeninthecoke.Meanwhile,thereleasinglawofNOxinthefluegasiscloselylinkedtotheruleofcokecombustion.AllthesecanbeconcludedthattheNOxinsinteringaremainfueltypeNOx.N2Owasdetectedin