燃煤初期碳烟生成的激光诱导白炽光LII诊断研究.docxVIP

中国工程热物理学会学术会议论文 中国工程热物理学会 学术会议论文 编号： 燃煤初期碳烟生成的激光诱导白炽光LII诊断研究 高琦1,李水清1,*,Diego Zabrodiec2,Reinhold Kneer2,姚强1 （1.清华大学能源与动力工程系 热科学与动力工程教育部重点实验室 北京 100084 中国 2.亚琛工业大学 传热传质研究中心 亚琛 52062 德国） (Tel Email：lishuiqing@mail.tsinghua.edu.cn) 摘 要：本文基于光学可视化Hencken平焰燃烧器系统平台，采用激光诱导白炽光（LII）方法对不同煤阶煤种燃烧初期产生的碳烟颗粒进行在线诊断。研究结果表明，高阶PH煤在燃烧初期产生的碳烟量明显高于低阶准东（Zhundong）煤。化学渗透热解模型计算结果证明这一现象主要由PH煤热解过程中较Zhundong煤更高的焦油产量所致。时间尺度分析表明，在1500 K，20% O2燃烧条件下，PH煤碳烟明显生成的特征时间（~20 ms）滞后于煤粉点火特征时间（~10 ms）和挥发分燃烧特征时间（~12 ms）。并随着气氛中氧气浓度的降低，碳烟生成的特征时间增加。通过建立简化的碳烟生成/氧化模型，进一步揭示了煤粉燃烧初期煤粉点火、挥发分燃烧和碳烟生成过程的内在物理联系。另外，与常规条件相比，富氧条件对煤粉燃烧初期碳烟生成存在抑制作用。 关键词：碳烟；激光诱导白炽光（LII）；Hencken燃烧器；时间尺度分析 Laser-Induced Incandescence (LII) Diagnostics on the Soot Formation in the Early Stage of Pulverized Coal Combustion Qi Gao1, Shuiqing Li1,*, Diego Zabrodiec2,Reinhold Kneer2,Qiang Yao1 1. Department of Energy and Power Engineering, Key Laboratory for Thermal Science and Power Engineering of Ministry of Education, Tsinghua University, Beijing, 100084, China 2. Institute of Heat and Mass Transfer, RWTH Aachen University, Augustinerbach 6, 52062 Aachen, Germany Tel: Email: lishuiqing@mail.tsinghua.edu.cn Abstract: In this work, we diagnosed the soot formation in the early stage of coal combustion with the laser-induced incandescence (LII) technique in an optically-accessible Hencken flat flame burner system. Results indicate that the combustion of high-rank PH coal yields a significantly higher amount of soot particles than that of low-rank Zhundong coal. It is mainly attributed to the higher tar production from PH coal according to the calculation results of chemical percolation devolatilization (CPD) model. Further time-scale analyses manifest that the appearance of soot particles (~20 ms) lags behind the ignition of coal particles (~10 ms) and combustion of released volatiles (~12 ms) in the condition of 1500 K and 20 % O2. Moreover, the characteristic time of soot formation is postponed as the increase of ambient oxyge