长沙地区水体蒸发中稳定同位素分馏实验和模拟分析.pdf

的下降的过程。而动力分馏模式模拟结果不仅全程与实测结果拟合较 好，而且能很好地模拟剩余水体稳定同位素比率波动的过程。 3 实测剩余水体蒸发线斜率冬春两季大于动力模拟蒸发线，夏 秋两季反之。说明在夏秋两季实际蒸发作用更明显，冬春两季水体蒸 发受到温度条件限制。平衡模式模拟的蒸发线斜率高于实测蒸发线和 动力模拟蒸发线斜率，与大气降水线接近，拟合程度不理想。动力模 拟蒸发线斜率与实测蒸发线斜率接近，夏秋季前者高于后者，冬春季 反之。 4 六组实验蒸发水体中过量氘d值随蒸发总体呈下降趋势，但 在出现降水时段过量氘d值会出现回升。从过量氘d值的下降平均速 度来看，夏季下降速度最高，秋季其次。冬春季过量氘d值下降速度 较慢。 5 大气水汽中62H和蒸发剩余水体中62H在降水时间出现同步 下降，证明了蒸发剩余水体中稳定同位素在降水时段受到大气水汽中 稳定同位素变化的影响。 关键词：长沙；蒸发实验；稳定同位素；模拟 万方数据 ABSTRACT isa inthewater onearthand Evaporationsignificant it progress cycle the ofstable between waterand impactsexchange isotopes evaporation in thevariationofstable in vaporatmosphere．Meanwhile isotopes wateris relatedtothe factorsand evaporationclosely meteorological extent．Winteriscoldandsummerishotin evaporation Changsha．The variationof inawholecouldbe 40。C．Affected temperatureyear nearly bymonsoon，theof alsocouldbe disparityhumidity water this in contextis tounderstandthe evaporationexperiments helpful fractionationlawofwaterstable indifferentweatherand isotope the contributionofstable fromwaterto isotopes arethebest to thestable fractionation experiments wayverify isotope theory． Basedonsix ofwater groups’observationevaporationexperiments， thecharacteristicsofstable variationin Paperanalyzed isotope waterandthe ofwaterstable variation evaporation relationship isotope and air fractionationmodel humidity．Usingequilibrium andkinetic fractionationmodelsimulatethevariationof waterstable evaporation and itwithmeasured October isotope 2014，the compare Value．During variation of waterstable andthevariationof evaporation isotopes vapor stable wereobserved mainresultsareas isotopes simultaneously．The follows： III 万方数据 ratioofstable in residualwaterisincreased 1 The isotopeevaporation withthedecreaseof residualwatermass．But along evaporation during theratioofstable in residualwaterwill evaporation precipitation isotope decline．Theratioofstable in residualwaterandair isotopeevaporation demonstrateda correlation． humidity negative simulationresultsof modelwellfi