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Depletion of λ-DNA near moving contact line.pdf
Journal of Non-Newtonian Fluid Mechanics 236 (2016) 50–62
Contents lists available at ScienceDirect
Journal of Non-Newtonian Fluid Mechanics
journal homepage: /locate/jnnfm
Depletion of λ-DNA near moving contact line
Hongrok Shin, Ki Wan Bong?, Chongyoup Kim??
Department of Chemical and Biological Engineering, Korea University, Anam-dong, Sungbuk-ku, Seoul 136-713, Korea
article info
Article history: Received 11 February 2016 Revised 25 August 2016 Accepted 25 August 2016 Available online 28 August 2016
Keywords: Contact line motion Migration Elasticity Elastic dumbbell model Inhomogeneous ?ow
abstract
An understanding of the contact line dynamics of viscoelastic liquids is essential for the successful ap-
plication of liquid processing methods in many industries. In this article, the contact line motion of a λ-
DNA solution is considered both experimentally and theoretically to understand the contact line motion
of polymeric solutions. Experimentally, by using ?uorescently tagged λ-DNAs in glycerin, the depletion of λ-DNA near the contact line is observed. The depletion length increases with time in a range near 10 μm. DNA fragments in glycerin did not show such a depletion region. The geometric exclusion of λDNA from the region cannot be the proper reason for the depletion because λ-DNA is in the stretched
state. It is suggested that the depletion region might be developed by the migration of polymers from the solid wall to the bulk due to the elasticity of polymers. In the theoretical study, the Stokes ?ow near the contact line region is solved analytically for a drop-spreading problem to obtain the inhomogeneous ?ow ?eld. Then, the motions of DNAs are considered in the ?ow using the FENE-P dumbbell model at the dilute limit. Two independent mechanisms of migration of the dumbbells were considered: migration due to wall-bead hydrodynamic interactions and the migration of stretched dumbbells in the inhomogeneous ?ow. It was found that the migration of stretched du
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