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The glassy state — Magnetically viewed from the frozen end.pdf

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The glassy state — Magnetically viewed from the frozen end.pdf

Journal of Non-Crystalline Solids 401 (2014) 66–72 Contents lists available at ScienceDirect Journal of Non-Crystalline Solids journal homepage: / locate/ jnoncrysol The glassy state — Magnetically viewed from the frozen end Giancarlo Jug a,c,d,?, Maksym Paliienko b, Silvia Bonfanti a a Dipartimento di Scienza ed Alta Tecnologia, Università dellInsubria, Via Valleggio 11, 22100 Como, Italy b Sumy State University, Rimskii-Korsakov St. 2, 40007 Sumy, Ukraine c INFN, Sezione di Pavia, Italy d IPCF, Sezione di Roma, Italy article info Article history: Received 16 September 2013 Received in revised form 5 December 2013 Available online 8 January 2014 Keywords: Crystalline-like ordering in glasses; Low temperature physics; Magnetic effects in non-magnetic glasses; Oxide and organic glasses (non-metallic); Tunneling systems in glasses abstract It is argued that the structure of real glasses, especially the multi-component ones, can be investigated at low temperatures by exploiting the existence of tunneling systems (TSs) in the glass which can be described by a suitable extension of the standard tunneling model (STM) as was proposed by one of us. Even the simplest glass – as already argued in 1921 and in 1937 by A.A. Lebedev – is likely to contain elementary crystallites (not yet crystals) embedded in a random network, and our work has shown that this statement is even more true in the case of phase-separating, multi-component glasses, solids containing network-modifying components in their chemical make-up. Using the concept of TSs speci?cally nesting within the crystallites, we describe how our extended TM can explain puzzling experiments in glasses at low temperatures and in the presence of a magnetic ?eld for a variety of amorphous insulators. The success of the theoretical analysis of a large number of experimental data con?rms the crystallite hypothesis, clari?es the nature of the TS and opens the way to a possible new form of spectroscopy for the amorphous solid st