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A kinetic model for the decolorization of C.I. Acid Yellow 23 by Fenton process.pdf

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A kinetic model for the decolorization of C.I. Acid Yellow 23 by Fenton process

Ao a ? K 1 c o b i m m o t d t a t r f e a w [ i 0 dJournal of Hazardous Materials 148 (2007) 98–102 A kinetic model for the decolorization of C.I. Acid Yellow 23 by Fenton process M.A. Behnajady ?, N. Modirshahla, F. Ghanbary Department of Applied Chemistry, Islamic Azad University, Tabriz Branch, P.O. Box 1655, Tabriz, Islamic Republic of Iran Received 8 November 2006; received in revised form 3 February 2007; accepted 5 February 2007 Available online 12 February 2007 bstract The decolorization of azo dye C.I. Acid Yellow 23 (AY23) by Fenton process was investigated. The decolorization rate is strongly dependent n the initial concentrations of the Fe2+ and H2O2. The optimum operational conditions were obtained at pH 3. A kinetic model has been developed to predict the decolorization of AY23 at different operational conditions by Fenton process. The model llows to simulate the system behavior involving the influence of hydrogen peroxide, Fe(II) and dye concentrations. 2007 Elsevier B.V. All rights reserved. ; Kin a o e f e p p w T h a F m [ H peywords: Advanced oxidation processes (AOPs); Fenton; C.I. Acid Yellow 23 . Introduction Synthetic dyes are the major industrial pollutants and water ontaminants [1–3]. Wastewater from textile, paper, and some ther industries contain residual dyes, which are not readily iodegradable. Azo dyes, the largest class of synthetic dyes used n food industries, are characterized by the presence of one or ore azo bonds (–N N–) in association with one or more aro- atic systems, which may also carry sulfonic acid groups. One f them is Tartrazine or C.I. Acid Yellow 23 an azo dye present in housands of foods and drugs. Many studies indicate that these yes are toxic or carcinogenic. If these colorants come into con- act along with certain drugs in the human body they can induce llergic and asthmatic reactions in sensitive people. An addi- ional difficulty is that, when present, these dyes are not normally emoved by conventional wastewater