Fabrication of Localized Surface Plasmon Resonance Fiber Probes Using Ionic Self-Assembled Gold Nanoparticles.docVIP

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Fabrication of Localized Surface Plasmon Resonance Fiber Probes Using Ionic Self-Assembled Gold Nanoparticles.doc

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Fabrication of Localized Surface Plasmon Resonance Fiber Probes Using Ionic Self-Assembled Gold Nanoparticles

Sensors 2010, 10, 6477-6487; doi:10.3390/s100706477 OPEN ACCESS sensors ISSN 1424-8220 /journal/sensors Article Fabrication of Localized Surface Plasmon Resonance Fiber Probes Using Ionic Self-Assembled Gold Nanoparticles Miao Wan 1,2, Pengfei Luo 1, Jiayi Jin 3, Jiong Xing 1, Zhiyong Wang 1,* and Stephen T. C. Wong 1,* 1 Bioengineering and Bioinformatics Program, The Methodist Hospital Research Institute, Weill Cornell Medical College, Houston, Texas 77030, USA; E-Mails: wmwhdz07@ (M.W.); PLuo@ (P.L.); JXing@ (J.X.) 2 College of Math and Physics, China University of Geoscience, Wuhan 430074, China 3 Department of Electrical Computer Engineering, Texas AM University, College Station, Texas 77844, USA; E-Mail: jjy2005@ (J.J.) * Author to whom correspondence should be addressed; E-Mails: Zhwang@ (Z.W.); STWong@ (S.T.W.) Received: 11 May 2010; in revised form: 8 June 2010 / Accepted: 21 June 2010 / Published: 1 July 2010 Abstract: An nm-thickness composite gold thin film consisting of gold nanoparticles and polyelectrolytes is fabricated through ionic self-assembled multilayers (ISAM) technique and is deposited on end-faces of optical fibers to construct localized surface plasmon resonance (LSPR) fiber probes. We demonstrate that the LSPR spectrum induced by ISAM gold films can be fine-tuned through the ISAM procedure. We investigate variations of reflection spectra of the probe with respect to the layer-by-layer adsorption of ISAMs onto end-faces of fibers, and study the spectral variation mechanism. Finally, we demonstrated using this fiber probe to detect the biotin-streptavidin bioconjugate pair. ISAM adsorbed on optical fibers potentially provides a simple, fast, robust, and low-cost, platform for LSPR biosensing applications. Keywords: localized surface plasmon resonance; ionic self-assembled multilayers; fiber optics; biosensors Sensors 2010, 10 6478 1. Introduction Localized surface plasmon resonance (LSPR)